In-gap spin excitations and finite triplet lifetimes in the dilute singlet ground state system SrCu(2-x)Mgx(BO3)2.
High resolution neutron scattering measurements on a single crystal of SrCu(2-x)Mgx(BO3)2 with x approximately 0.05 reveal the presence of new spin excitations within the gap of this quasi-two-dimensional, singlet ground state system. The application of a magnetic field induces Zeeman-split states associated with S=1/2 unpaired spins which are antiferromagnetically correlated with the bulk singlet. Substantial broadening of both the one- and two-triplet excitations in the doped single crystal is observed, as compared with pure SrCu2(BO3)2. Theoretical calculations using a variational algorithm and a single quenched magnetic vacancy on an infinite lattice are shown to qualitatively account for these effects.
Haravifard, S; Dunsiger, SR; El Shawish, S; Gaulin, BD; Dabkowska, HA; Telling, MT; Perring, TG; Bonca, J
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