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MAPbI3 Solar Cells with Absorber Deposited by Resonant Infrared Matrix-Assisted Pulsed Laser Evaporation

Publication ,  Journal Article
Dunlap-Shohl, WA; Barraza, ET; Barrette, A; Gundogdu, K; Stiff-Roberts, AD; Mitzi, DB
Published in: ACS Energy Letters
February 9, 2018

Resonant infrared, matrix-assisted pulsed laser evaporation (RIR-MAPLE) is a gentle thin-film deposition technique that combines the facile chemical control of solution processing with the growth control of vapor-phase deposition, yet one that has not been widely applied to crystalline organic-inorganic hybrid materials. In this work, we investigate the optoelectronic quality of RIR-MAPLE-deposited CH3NH3PbI3 (MAPbI3) perovskite films and report on the fabrication of perovskite solar cells in which the absorber is deposited by RIR-MAPLE. We find the composition, morphology, and optical properties of these perovskite films to be comparable to those produced by more conventional methods, such as spin coating. The champion device reaches a stabilized power conversion efficiency of over 12%, a high value for perovskite solar cells deposited by a laser ablation process, highlighting the ability of this new technique to produce device-quality films.

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Published In

ACS Energy Letters

DOI

EISSN

2380-8195

Publication Date

February 9, 2018

Volume

3

Issue

2

Start / End Page

270 / 275

Related Subject Headings

  • 40 Engineering
  • 34 Chemical sciences
 

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Dunlap-Shohl, W. A., Barraza, E. T., Barrette, A., Gundogdu, K., Stiff-Roberts, A. D., & Mitzi, D. B. (2018). MAPbI3 Solar Cells with Absorber Deposited by Resonant Infrared Matrix-Assisted Pulsed Laser Evaporation. ACS Energy Letters, 3(2), 270–275. https://doi.org/10.1021/acsenergylett.7b01144
Dunlap-Shohl, W. A., E. T. Barraza, A. Barrette, K. Gundogdu, A. D. Stiff-Roberts, and D. B. Mitzi. “MAPbI3 Solar Cells with Absorber Deposited by Resonant Infrared Matrix-Assisted Pulsed Laser Evaporation.” ACS Energy Letters 3, no. 2 (February 9, 2018): 270–75. https://doi.org/10.1021/acsenergylett.7b01144.
Dunlap-Shohl WA, Barraza ET, Barrette A, Gundogdu K, Stiff-Roberts AD, Mitzi DB. MAPbI3 Solar Cells with Absorber Deposited by Resonant Infrared Matrix-Assisted Pulsed Laser Evaporation. ACS Energy Letters. 2018 Feb 9;3(2):270–5.
Dunlap-Shohl, W. A., et al. “MAPbI3 Solar Cells with Absorber Deposited by Resonant Infrared Matrix-Assisted Pulsed Laser Evaporation.” ACS Energy Letters, vol. 3, no. 2, Feb. 2018, pp. 270–75. Scopus, doi:10.1021/acsenergylett.7b01144.
Dunlap-Shohl WA, Barraza ET, Barrette A, Gundogdu K, Stiff-Roberts AD, Mitzi DB. MAPbI3 Solar Cells with Absorber Deposited by Resonant Infrared Matrix-Assisted Pulsed Laser Evaporation. ACS Energy Letters. 2018 Feb 9;3(2):270–275.
Journal cover image

Published In

ACS Energy Letters

DOI

EISSN

2380-8195

Publication Date

February 9, 2018

Volume

3

Issue

2

Start / End Page

270 / 275

Related Subject Headings

  • 40 Engineering
  • 34 Chemical sciences