Femtosecond phase-coherent two-dimensional spectroscopy.
Publication
, Journal Article
Tian, P; Keusters, D; Suzaki, Y; Warren, WS
Published in: Science (New York, N.Y.)
June 2003
Femtosecond phase-coherent two-dimensional (2D) spectroscopy has been experimentally demonstrated as the direct optical analog of 2D nuclear magnetic resonance. An acousto-optic pulse shaper created a collinear three-pulse sequence with well-controlled and variable interpulse delays and phases,which interacted with a model atomic system of rubidium vapor. The desired nonlinear polarization was selected by phase cycling (coadding experimental results obtained with different interpulse phases). This method may enhance our ability to probe the femtosecond structural dynamics of macromolecules.
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Published In
Science (New York, N.Y.)
DOI
EISSN
1095-9203
ISSN
0036-8075
Publication Date
June 2003
Volume
300
Issue
5625
Start / End Page
1553 / 1555
Related Subject Headings
- Time Factors
- Spectrum Analysis
- Rubidium
- Photons
- Optics and Photonics
- Molecular Structure
- Mathematics
- Magnetic Resonance Spectroscopy
- Lasers
- General Science & Technology
Citation
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Chicago
ICMJE
MLA
NLM
Tian, P., Keusters, D., Suzaki, Y., & Warren, W. S. (2003). Femtosecond phase-coherent two-dimensional spectroscopy. Science (New York, N.Y.), 300(5625), 1553–1555. https://doi.org/10.1126/science.1083433
Tian, Peifang, Dorine Keusters, Yoshifumi Suzaki, and Warren S. Warren. “Femtosecond phase-coherent two-dimensional spectroscopy.” Science (New York, N.Y.) 300, no. 5625 (June 2003): 1553–55. https://doi.org/10.1126/science.1083433.
Tian P, Keusters D, Suzaki Y, Warren WS. Femtosecond phase-coherent two-dimensional spectroscopy. Science (New York, NY). 2003 Jun;300(5625):1553–5.
Tian, Peifang, et al. “Femtosecond phase-coherent two-dimensional spectroscopy.” Science (New York, N.Y.), vol. 300, no. 5625, June 2003, pp. 1553–55. Epmc, doi:10.1126/science.1083433.
Tian P, Keusters D, Suzaki Y, Warren WS. Femtosecond phase-coherent two-dimensional spectroscopy. Science (New York, NY). 2003 Jun;300(5625):1553–1555.
Published In
Science (New York, N.Y.)
DOI
EISSN
1095-9203
ISSN
0036-8075
Publication Date
June 2003
Volume
300
Issue
5625
Start / End Page
1553 / 1555
Related Subject Headings
- Time Factors
- Spectrum Analysis
- Rubidium
- Photons
- Optics and Photonics
- Molecular Structure
- Mathematics
- Magnetic Resonance Spectroscopy
- Lasers
- General Science & Technology