Polyethylenimine-enhanced electrocatalytic reduction of CO2 to formate at nitrogen-doped carbon nanomaterials
Publication
, Journal Article
Zhang, S; Kang, P; Ubnoske, S; Brennaman, MK; Song, N; House, RL; Glass, JT; Meyer, TJ
Published in: Journal of the American Chemical Society
June 4, 2014
Nitrogen-doped carbon nanotubes are selective and robust electrocatalysts for CO2 reduction to formate in aqueous media without the use of a metal catalyst. Polyethylenimine (PEI) functions as a co-catalyst by significantly reducing catalytic overpotential and increasing current density and efficiency. The co-catalysis appears to help in stabilizing the singly reduced intermediate CO2•- and concentrating CO 2 in the PEI overlayer. © 2014 American Chemical Society.
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Published In
Journal of the American Chemical Society
DOI
EISSN
1520-5126
ISSN
0002-7863
Publication Date
June 4, 2014
Volume
136
Issue
22
Start / End Page
7845 / 7848
Related Subject Headings
- General Chemistry
- 40 Engineering
- 34 Chemical sciences
- 03 Chemical Sciences
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Zhang, S., Kang, P., Ubnoske, S., Brennaman, M. K., Song, N., House, R. L., … Meyer, T. J. (2014). Polyethylenimine-enhanced electrocatalytic reduction of CO2 to formate at nitrogen-doped carbon nanomaterials. Journal of the American Chemical Society, 136(22), 7845–7848. https://doi.org/10.1021/ja5031529
Zhang, S., P. Kang, S. Ubnoske, M. K. Brennaman, N. Song, R. L. House, J. T. Glass, and T. J. Meyer. “Polyethylenimine-enhanced electrocatalytic reduction of CO2 to formate at nitrogen-doped carbon nanomaterials.” Journal of the American Chemical Society 136, no. 22 (June 4, 2014): 7845–48. https://doi.org/10.1021/ja5031529.
Zhang S, Kang P, Ubnoske S, Brennaman MK, Song N, House RL, et al. Polyethylenimine-enhanced electrocatalytic reduction of CO2 to formate at nitrogen-doped carbon nanomaterials. Journal of the American Chemical Society. 2014 Jun 4;136(22):7845–8.
Zhang, S., et al. “Polyethylenimine-enhanced electrocatalytic reduction of CO2 to formate at nitrogen-doped carbon nanomaterials.” Journal of the American Chemical Society, vol. 136, no. 22, June 2014, pp. 7845–48. Scopus, doi:10.1021/ja5031529.
Zhang S, Kang P, Ubnoske S, Brennaman MK, Song N, House RL, Glass JT, Meyer TJ. Polyethylenimine-enhanced electrocatalytic reduction of CO2 to formate at nitrogen-doped carbon nanomaterials. Journal of the American Chemical Society. 2014 Jun 4;136(22):7845–7848.
Published In
Journal of the American Chemical Society
DOI
EISSN
1520-5126
ISSN
0002-7863
Publication Date
June 4, 2014
Volume
136
Issue
22
Start / End Page
7845 / 7848
Related Subject Headings
- General Chemistry
- 40 Engineering
- 34 Chemical sciences
- 03 Chemical Sciences