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Formation dynamics of excitons and temporal behaviors of Fano resonance due to the exciton-impurity-phonon configuration interaction in ZnO.

Publication ,  Journal Article
Zheng, CC; Xu, SJ; Ning, JQ; Chen, YN; Li, BK; Wang, JN; Che, CM
Published in: The journal of physical chemistry. A
January 2012

Formation dynamics of free and neutral donor bound excitons (FX and D(0)X) in a high quality ZnO single crystal are studied by means of time-resolved photoluminescence (TRPL) at various temperatures. At low-temperatures, FX and D(0)X formation times are determined to be ~5 and ~10 ps, respectively, by fitting the rise process with the Boltzmann sigmoidal function. Temporal information of FX- and D(0)X-longitudinal optical (LO) phonon coupling is also acquired by measuring TRPL spectra of the first-order LO phonon-assisted FX and D(0)X transitions. In particular, interesting time evolution of luminescence intensity in the Fano resonance region due to the configuration interaction of exciton-impurity-phonon is explored.

Duke Scholars

Published In

The journal of physical chemistry. A

DOI

EISSN

1520-5215

ISSN

1089-5639

Publication Date

January 2012

Volume

116

Issue

1

Start / End Page

381 / 385

Related Subject Headings

  • 5102 Atomic, molecular and optical physics
  • 3407 Theoretical and computational chemistry
  • 3406 Physical chemistry
  • 0307 Theoretical and Computational Chemistry
  • 0306 Physical Chemistry (incl. Structural)
  • 0202 Atomic, Molecular, Nuclear, Particle and Plasma Physics
 

Citation

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Zheng, C. C., Xu, S. J., Ning, J. Q., Chen, Y. N., Li, B. K., Wang, J. N., & Che, C. M. (2012). Formation dynamics of excitons and temporal behaviors of Fano resonance due to the exciton-impurity-phonon configuration interaction in ZnO. The Journal of Physical Chemistry. A, 116(1), 381–385. https://doi.org/10.1021/jp209919n
Zheng, C. C., S. J. Xu, J. Q. Ning, Y. N. Chen, B. K. Li, J. N. Wang, and C. M. Che. “Formation dynamics of excitons and temporal behaviors of Fano resonance due to the exciton-impurity-phonon configuration interaction in ZnO.The Journal of Physical Chemistry. A 116, no. 1 (January 2012): 381–85. https://doi.org/10.1021/jp209919n.
Zheng CC, Xu SJ, Ning JQ, Chen YN, Li BK, Wang JN, et al. Formation dynamics of excitons and temporal behaviors of Fano resonance due to the exciton-impurity-phonon configuration interaction in ZnO. The journal of physical chemistry A. 2012 Jan;116(1):381–5.
Zheng, C. C., et al. “Formation dynamics of excitons and temporal behaviors of Fano resonance due to the exciton-impurity-phonon configuration interaction in ZnO.The Journal of Physical Chemistry. A, vol. 116, no. 1, Jan. 2012, pp. 381–85. Epmc, doi:10.1021/jp209919n.
Zheng CC, Xu SJ, Ning JQ, Chen YN, Li BK, Wang JN, Che CM. Formation dynamics of excitons and temporal behaviors of Fano resonance due to the exciton-impurity-phonon configuration interaction in ZnO. The journal of physical chemistry A. 2012 Jan;116(1):381–385.
Journal cover image

Published In

The journal of physical chemistry. A

DOI

EISSN

1520-5215

ISSN

1089-5639

Publication Date

January 2012

Volume

116

Issue

1

Start / End Page

381 / 385

Related Subject Headings

  • 5102 Atomic, molecular and optical physics
  • 3407 Theoretical and computational chemistry
  • 3406 Physical chemistry
  • 0307 Theoretical and Computational Chemistry
  • 0306 Physical Chemistry (incl. Structural)
  • 0202 Atomic, Molecular, Nuclear, Particle and Plasma Physics