Matthew L Becker | Scholars@Duke

Matthew L Becker
Hugo L. Blomquist Distinguished Professor of Chemistry

The Becker Laboratory for Functional Biomaterials is a multidisciplinary organic materials group working at the interface of chemistry, organic materials and medicine. We are developing families of degradable polymers with highly tunable physical and biological properties that are being applied to unmet needs in bone, soft tissue, neural and vascular tissue engineering. We are also actively engaged in additive manufacturing and the development of custom inks that are enabling unique solutions to challenging design paradigms in biomaterials and drug delivery.

Current Research Interests

Polymer chemistry; bioconjugate chemistry; molecular imaging and additive manufacturing; materials for bone, soft tissue, neural and vascular tissue engineering; drug and protein delivery; degradable materials for flexible electronics

Current Appointments & Affiliations

Hugo L. Blomquist Distinguished Professor of Chemistry, Chemistry, Trinity College of Arts & Sciences 2020
Professor of Chemistry, Chemistry, Trinity College of Arts & Sciences 2019
Professor of Mechanical Engineering and Material Science, Thomas Lord Department of Mechanical Engineering and Materials Science, Pratt School of Engineering 2019
Professor of Biomedical Engineering, Biomedical Engineering, Pratt School of Engineering 2019

Contact Information

B120 Levine Science Res Center, 308 Research Drive, Durham, NC 27708
B120 Levine Science Res Center, 308 Research Drive, Durham, NC 27708
matthew.l.becker@duke.edu (919) 681-3812
Becker Research Group

Background
Education, Training, & Certifications
- Ph.D., Washington University in St. Louis 2003
- M.A., Washington University in St. Louis 2000
- B.S., Northwest Missouri State University 1998
Previous Appointments & Affiliations
- Scholar In Residence of Chemistry, Chemistry, Trinity College of Arts & Sciences 2019
Recognition
In the News
- JAN 26, 2022 Office of Translation & Commercialization
  
  Sweet Science: Researchers Develop Recyclable Plastics Based on Sugars
- JAN 11, 2021
  
  Post-Surgical Patch Releases Non-Opioid Painkiller Directly to the Wound
- APR 14, 2020
  
  Duke Awards 29 University Distinguished Professorships
- OCT 15, 2019 Duke Stories
  
  New Faculty, Bold Thinking
Awards & Honors
Expertise
Subject Headings
- Muser Mentor
Research
Selected Grants
- University Training Program in Biomolecular and Tissue Engineering awarded by National Institutes of Health 1994 - 2027
- Synergistic Enhancement of Peripheral Nerve Defect Repair using Peptide Functionalized Aligned Nanofiber Conduits awarded by National Institutes of Health 2022 - 2027
- Resorbable, Phsophorylated Poly(ester urea) Surgical Adhesive to Enhance Fracture Healing awarded by National Institutes of Health 2021 - 2026
- Pain Management in Critical Combat Casualty Environments using Resorbable Poly(ester urea) Films for Sustained Delivery of Meloxicam and Bupivacaine awarded by United States Army Medical Research Acquisition Activity 2022 - 2026
- RESORBABLE WATER BARRIER MATERIALS AND MACHINE LEARNING-DIRECTED SYNTHESIS awarded by Avient Corporation 2022 - 2025
- Modified Lens Fluids and Materials awarded by Adaptilens, LLC 2020 - 2023
- Tethered Ligands for Craniofacial Bone Tissue Engineering awarded by Ohio State University 2021 - 2023
- FDA-SIR: Designing for Degradation: A framework for Predicting in vivo Degradation and Mechanical Property Changes in Degradable Polymers awarded by National Science Foundation 2021 - 2022
- An Elastomeric Composite Hernia Mesh, Termed Safe Mesh, to Prevent Post-Operative Adhesions awarded by North Carolina Biotechnology Center 2021 - 2022
- Trust in Flexible Electronic Devices and Additive Manufacturing awarded by University of Akron 2019 - 2021
External Relationships
- 21MedTech
- Adaptilens, LLC
- Artelon
Publications & Artistic Works
Selected Publications
- Academic Articles
  - Kirillova, Alina, Taylor R. Yeazel, Ken Gall, and Matthew L. Becker. “Thiol-Based Three-Dimensional Printing of Fully Degradable Poly(propylene fumarate) Star Polymers.” Acs Applied Materials & Interfaces 14, no. 34 (August 2022): 38436–47. https://doi.org/10.1021/acsami.2c06553.
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  - Cavanaugh, McKay, Darya Asheghali, Cecilia M. Motta, Elena Silantyeva, Shantanu P. Nikam, Matthew L. Becker, and Rebecca K. Willits. “Influence of Touch-Spun Nanofiber Diameter on Contact Guidance during Peripheral Nerve Repair.” Biomacromolecules 23, no. 6 (June 2022): 2635–46. https://doi.org/10.1021/acs.biomac.2c00379.
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  - Petersen, Shannon R., Jiayi Yu, Taylor R. Yeazel, Garrett Bass, Aslan Alamdari, and Matthew L. Becker. “Degradable, Photochemically Printable Poly(propylene fumarate)-Based ABA Triblock Elastomers.” Biomacromolecules 23, no. 6 (June 2022): 2388–95. https://doi.org/10.1021/acs.biomac.2c00151.
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  - Shin, Yongjun, and Matthew L. Becker. “Gradient versus End-Capped Degradable Polymer Sequence Variations Result in Stiff to Elastic Photochemically 3D-Printed Substrates.” Biomacromolecules 23, no. 5 (May 2022): 2106–15. https://doi.org/10.1021/acs.biomac.2c00103.
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  - Stubbs, Connor J., Joshua C. Worch, Hannah Prydderch, Zilu Wang, Robert T. Mathers, Andrey V. Dobrynin, Matthew L. Becker, and Andrew P. Dove. “Correction to "Sugar-Based Polymers with Stereochemistry Dependent Degradability and Mechanical Properties".” Journal of the American Chemical Society 144, no. 17 (May 2022): 7949–50. https://doi.org/10.1021/jacs.2c03696.
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  - Petersen, Shannon R., Hannah Prydderch, Joshua C. Worch, Connor J. Stubbs, Zilu Wang, Jiayi Yu, Maria C. Arno, Andrey V. Dobrynin, Matthew L. Becker, and Andrew P. Dove. “Ultra-Tough Elastomers from Stereochemistry-Directed Hydrogen Bonding in Isosorbide-Based Polymers.” Angewandte Chemie (International Ed. in English) 61, no. 17 (April 2022): e202115904. https://doi.org/10.1002/anie.202115904.
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  - Hsu, Yen-Hao, Derek Luong, Darya Asheghali, Andrew P. Dove, and Matthew L. Becker. “Shape Memory Behavior of Biocompatible Polyurethane Stereoelastomers Synthesized via Thiol-Yne Michael Addition.” Biomacromolecules 23, no. 3 (March 2022): 1205–13. https://doi.org/10.1021/acs.biomac.1c01473.
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  - Roesner, E. K., D. Asheghali, A. Kirillova, M. J. Strauss, A. M. Evans, M. L. Becker, and W. R. Dichtel. “Arene-perfluoroarene interactions confer enhanced mechanical properties to synthetic nanotubes.” Chemical Science 13, no. 8 (February 28, 2022): 2475–80. https://doi.org/10.1039/d1sc05932g.
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  - Stubbs, Connor J., Joshua C. Worch, Hannah Prydderch, Zilu Wang, Robert T. Mathers, Andrey V. Dobrynin, Matthew L. Becker, and Andrew P. Dove. “Sugar-Based Polymers with Stereochemistry-Dependent Degradability and Mechanical Properties.” Journal of the American Chemical Society 144, no. 3 (January 2022): 1243–50. https://doi.org/10.1021/jacs.1c10278.
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  - Zhao, J., H. Tong, A. Kirillova, W. J. Koshut, A. Malek, N. C. Brigham, M. L. Becker, K. Gall, and B. J. Wiley. “A Synthetic Hydrogel Composite with a Strength and Wear Resistance Greater than Cartilage.” Advanced Functional Materials, January 1, 2022. https://doi.org/10.1002/adfm.202205662.
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  - Khalfa, Anissa L., Matthew L. Becker, and Andrew P. Dove. “Stereochemistry-Controlled Mechanical Properties and Degradation in 3D-Printable Photosets.” Journal of the American Chemical Society 143, no. 42 (October 2021): 17510–16. https://doi.org/10.1021/jacs.1c06960.
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  - Endres, K. J., R. A. Dilla, M. L. Becker, and C. Wesdemiotis. “Poly(ethylene glycol) Hydrogel Crosslinking Chemistries Identified via Atmospheric Solids Analysis Probe Mass Spectrometry.” Macromolecules 54, no. 17 (September 14, 2021): 7754–64. https://doi.org/10.1021/acs.macromol.1c00765.
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  - Becker, Matthew L., and Jason A. Burdick. “Introduction: Polymeric Biomaterials.” Chemical Reviews 121, no. 18 (September 2021): 10789–91. https://doi.org/10.1021/acs.chemrev.1c00354.
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  - Kirillova, Alina, Taylor R. Yeazel, Darya Asheghali, Shannon R. Petersen, Sophia Dort, Ken Gall, and Matthew L. Becker. “Fabrication of Biomedical Scaffolds Using Biodegradable Polymers.” Chemical Reviews 121, no. 18 (September 2021): 11238–304. https://doi.org/10.1021/acs.chemrev.0c01200.
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  - Karayilan, M., J. Vakil, D. Fowler, M. L. Becker, and C. T. Cox. “Zooming in on polymer chemistry and designing synthesis of high sulfur-content polymers for virtual undergraduate laboratory experiment.” Journal of Chemical Education 98, no. 6 (June 8, 2021): 2062–73. https://doi.org/10.1021/acs.jchemed.1c00105.
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  - Hsu, Y. H., A. P. Dove, and M. L. Becker. “Crosslinked Internal Alkyne-Based Stereo Elastomers: Polymers with Tunable Mechanical Properties.” Macromolecules 54, no. 10 (May 25, 2021): 4649–57. https://doi.org/10.1021/acs.macromol.1c00246.
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  - Le Fer, G., R. A. Dilla, Z. Wang, J. King, S. S. C. Chuang, and M. L. Becker. “Clustering and Hierarchical Organization of 3D Printed Poly(propylene fumarate)- block-PEG- block-poly(propylene fumarate) ABA Triblock Copolymer Hydrogels.” Macromolecules 54, no. 7 (April 13, 2021): 3458–68. https://doi.org/10.1021/acs.macromol.1c00132.
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  - Brigham, Natasha C., Ru-Rong Ji, and Matthew L. Becker. “Degradable polymeric vehicles for postoperative pain management.” Nat Commun 12, no. 1 (March 1, 2021): 1367. https://doi.org/10.1038/s41467-021-21438-3.
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  - Bass, G. F., Y. Shin, and M. L. Becker. “Regio-Random Clemmensen Reduction of Biodegradable Polyesters for Photochemically Triggered 3D Printing.” Macromolecules 54, no. 3 (February 9, 2021): 1273–80. https://doi.org/10.1021/acs.macromol.0c02729.
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  - Karayilan, Metin, Liane Clamen, and Matthew L. Becker. “Polymeric Materials for Eye Surface and Intraocular Applications.” Biomacromolecules 22, no. 2 (February 2021): 223–61. https://doi.org/10.1021/acs.biomac.0c01525.
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  - Brigham, Natasha C., Rebecca Nofsinger, Xin Luo, Nathan Z. Dreger, Alexandra K. Abel, Tiffany P. Gustafson, Seth P. Forster, Andre Hermans, Ru-Rong Ji, and Matthew L. Becker. “Controlled release of etoricoxib from poly(ester urea) films for post-operative pain management.” J Control Release 329 (January 10, 2021): 316–27. https://doi.org/10.1016/j.jconrel.2020.11.052.
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  - Karayilan, M., S. M. McDonald, A. J. Bahnick, K. M. Godwin, Y. M. Chan, and M. L. Becker. “Reassessing Undergraduate Polymer Chemistry Laboratory Experiments for Virtual Learning Environments.” Journal of Chemical Education, January 1, 2021. https://doi.org/10.1021/acs.jchemed.1c01259.
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  - Wandel, Mary Beth, Craig A. Bell, Jiayi Yu, Maria C. Arno, Nathan Z. Dreger, Yen-Hao Hsu, Anaïs Pitto-Barry, Joshua C. Worch, Andrew P. Dove, and Matthew L. Becker. “Concomitant control of mechanical properties and degradation in resorbable elastomer-like materials using stereochemistry and stoichiometry for soft tissue engineering.” Nature Communications 12, no. 1 (January 2021): 446. https://doi.org/10.1038/s41467-020-20610-5.
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  - Tutoni, G., and M. L. Becker. “Underexplored Stereocomplex Polymeric Scaffolds with Improved Thermal and Mechanical Properties.” Macromolecules 53, no. 23 (December 8, 2020): 10303–14. https://doi.org/10.1021/acs.macromol.0c01468.
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  - Sayko, R., Z. Wang, H. Liang, M. L. Becker, and A. V. Dobrynin. “Degradation of Block Copolymer Films Confined in Elastic Media: Molecular Dynamics Simulations.” Macromolecules 53, no. 21 (November 10, 2020): 9460–69. https://doi.org/10.1021/acs.macromol.0c01795.
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  - Yeazel, Taylor R., and Matthew L. Becker. “Advancing Toward 3D Printing of Bioresorbable Shape Memory Polymer Stents.” Biomacromolecules 21, no. 10 (October 2020): 3957–65. https://doi.org/10.1021/acs.biomac.0c01082.
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  - Nikam, Shantanu P., Karissa Nettleton, Jeffrey I. Everitt, Hazel A. Barton, and Matthew L. Becker. “Antibiotic eluting poly(ester urea) films for control of a model cardiac implantable electronic device infection.” Acta Biomater 111 (July 15, 2020): 65–79. https://doi.org/10.1016/j.actbio.2020.04.025.
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  - Nikam, Shantanu P., Peiru Chen, Karissa Nettleton, Yen-Hao Hsu, and Matthew L. Becker. “Zwitterion Surface-Functionalized Thermoplastic Polyurethane for Antifouling Catheter Applications.” Biomacromolecules 21, no. 7 (July 2020): 2714–25. https://doi.org/10.1021/acs.biomac.0c00456.
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  - Worch, Joshua C., Andrew C. Weems, Jiayi Yu, Maria C. Arno, Thomas R. Wilks, Robert T. R. Huckstepp, Rachel K. O’Reilly, Matthew L. Becker, and Andrew P. Dove. “Elastomeric polyamide biomaterials with stereochemically tuneable mechanical properties and shape memory.” Nature Communications 11, no. 1 (June 2020): 3250. https://doi.org/10.1038/s41467-020-16945-8.
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  - Shin, Y., and M. L. Becker. “Alternating ring-opening copolymerization of epoxides with saturated and unsaturated cyclic anhydrides: Reduced viscosity poly(propylene fumarate) oligomers for use in cDLP 3D printing.” Polymer Chemistry 11, no. 19 (May 21, 2020): 3313–21. https://doi.org/10.1039/d0py00453g.
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  - Le Fer, Gaëlle, and Matthew L. Becker. “4D Printing of Resorbable Complex Shape-Memory Poly(propylene fumarate) Star Scaffolds.” Acs Applied Materials & Interfaces 12, no. 20 (May 2020): 22444–52. https://doi.org/10.1021/acsami.0c01444.
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  - Zhu, T., Y. Yang, L. Zheng, L. Liu, M. L. Becker, and X. Gong. “Solution-Processed Flexible Broadband Photodetectors with Solution-Processed Transparent Polymeric Electrode.” Advanced Functional Materials 30, no. 15 (April 1, 2020). https://doi.org/10.1002/adfm.201909487.
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  - Sayko, R., Z. Wang, H. Liang, M. L. Becker, and A. V. Dobrynin. “Degradation of Films of Block Copolymers: Molecular Dynamics Simulations.” Macromolecules 53, no. 4 (February 25, 2020): 1270–80. https://doi.org/10.1021/acs.macromol.9b02446.
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  - Chen, K., S. P. Nikam, Z. K. Zander, Y. H. Hsu, N. Z. Dreger, M. Cakmak, and M. L. Becker. “Continuous Fabrication of Antimicrobial Nanofiber Mats Using Post-Electrospinning Functionalization for Roll-to-Roll Scale-Up.” Acs Applied Polymer Materials 2, no. 2 (February 14, 2020): 304–16. https://doi.org/10.1021/acsapm.9b00798.
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  - Abel, Alexandra K., Nathan Z. Dreger, Karissa Nettleton, Tiffany P. Gustafson, Seth P. Forster, and Matthew L. Becker. “Amino Acid-Based Poly(ester urea)s as a Matrix for Extended Release of Entecavir.” Biomacromolecules 21, no. 2 (February 2020): 946–54. https://doi.org/10.1021/acs.biomac.9b01586.
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  - Stubbs, C. J., J. C. Worch, H. Prydderch, M. L. Becker, and A. P. Dove. “Unsaturated Poly(ester-urethanes) with Stereochemically Dependent Thermomechanical Properties.” Macromolecules 53, no. 1 (January 14, 2020): 174–81. https://doi.org/10.1021/acs.macromol.9b01700.
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  - Wang, K., L. Zheng, T. Zhu, L. Liu, M. L. Becker, and X. Gong. “High performance perovskites solar cells by hybrid perovskites co-crystallized with poly(ethylene oxide).” Nano Energy 67 (January 1, 2020). https://doi.org/10.1016/j.nanoen.2019.104229.
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  - Kleinfehn, Alex P., Jan A. Lammel Lindemann, Ali Razvi, Phinu Philip, Katelyn Richardson, Karissa Nettleton, Matthew L. Becker, and David Dean. “Modulating Bioglass Concentration in 3D Printed Poly(propylene fumarate) Scaffolds for Post-Printing Functionalization with Bioactive Functional Groups.” Biomacromolecules 20, no. 12 (December 2019): 4345–52. https://doi.org/10.1021/acs.biomac.9b00941.
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  - Silantyeva, Elena A., Rebecca K. Willits, and Matthew L. Becker. “Postfabrication Tethering of Molecular Gradients on Aligned Nanofibers of Functional Poly(ε-caprolactone)s.” Biomacromolecules 20, no. 12 (December 2019): 4494–4501. https://doi.org/10.1021/acs.biomac.9b01264.
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  - Dreger, Nathan Z., Zachary K. Zander, Yen-Hao Hsu, Derek Luong, Peiru Chen, Nancy Le, Trenton Parsell, et al. “Zwitterionic amino acid-based Poly(ester urea)s suppress adhesion formation in a rat intra-abdominal cecal abrasion model.” Biomaterials 221 (November 2019): 119399. https://doi.org/10.1016/j.biomaterials.2019.119399.
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  - Strauss, Michael J., Darya Asheghali, Austin M. Evans, Rebecca L. Li, Anton D. Chavez, Chao Sun, Matthew L. Becker, and William R. Dichtel. “Cooperative Self‐Assembly of Pyridine‐2,6‐Diimine‐Linked Macrocycles into Mechanically Robust Nanotubes.” Angewandte Chemie 131, no. 41 (October 7, 2019): 14850–56. https://doi.org/10.1002/ange.201907668.
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  - Guerra, Antonio J., Jan Lammel-Lindemann, Alex Katko, Alex Kleinfehn, Ciro A. Rodriguez, Luiz H. Catalani, Matthew L. Becker, Joaquim Ciurana, and David Dean. “Optimization of photocrosslinkable resin components and 3D printing process parameters.” Acta Biomaterialia 97 (October 2019): 154–61. https://doi.org/10.1016/j.actbio.2019.07.045.
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  - Motta, Cecilia M. M., Kevin J. Endres, Chrys Wesdemiotis, Rebecca K. Willits, and Matthew L. Becker. “Enhancing Schwann cell migration using concentration gradients of laminin-derived peptides.” Biomaterials 218 (October 2019): 119335. https://doi.org/10.1016/j.biomaterials.2019.119335.
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  - Strauss, Michael J., Darya Asheghali, Austin M. Evans, Rebecca L. Li, Anton D. Chavez, Chao Sun, Matthew L. Becker, and William R. Dichtel. “Cooperative Self-Assembly of Pyridine-2,6-Diimine-Linked Macrocycles into Mechanically Robust Nanotubes.” Angewandte Chemie (International Ed. in English) 58, no. 41 (October 2019): 14708–14. https://doi.org/10.1002/anie.201907668.
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  - Le Fer, G., Y. Luo, and M. L. Becker. “Poly(propylene fumarate) stars, using architecture to reduce the viscosity of 3D printable resins.” Polymer Chemistry 10, no. 34 (September 14, 2019): 4655–64. https://doi.org/10.1039/c9py00738e.
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  - Nettleton, Karissa, Derek Luong, Alex P. Kleinfehn, Laura Savariau, Christopher Premanandan, and Matthew L. Becker. “Molecular Mass-Dependent Resorption and Bone Regeneration of 3D Printed PPF Scaffolds in a Critical-Sized Rat Cranial Defect Model.” Advanced Healthcare Materials 8, no. 17 (September 2019): e1900646. https://doi.org/10.1002/adhm.201900646.
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  - Worch, J. C., H. Prydderch, S. Jimaja, P. Bexis, M. L. Becker, and A. P. Dove. “Stereochemical enhancement of polymer properties.” Nature Reviews Chemistry 3, no. 9 (September 1, 2019): 514–35. https://doi.org/10.1038/s41570-019-0117-z.
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  - Cai, Zhongyu, Yong Wan, Matthew L. Becker, Yun-Ze Long, and David Dean. “Poly(propylene fumarate)-based materials: Synthesis, functionalization, properties, device fabrication and biomedical applications.” Biomaterials 208 (July 2019): 45–71. https://doi.org/10.1016/j.biomaterials.2019.03.038.
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  - Xia, Xuhui, Garrett Bass, Matthew L. Becker, and Bryan D. Vogt. “Tuning Cooperative Assembly with Bottlebrush Block Co-polymers for Porous Metal Oxide Films Using Solvent Mixtures.” Langmuir : The Acs Journal of Surfaces and Colloids 35, no. 29 (July 2019): 9572–83. https://doi.org/10.1021/acs.langmuir.9b01363.
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  - Luo, Yuanyuan, Gaëlle Le Fer, David Dean, and Matthew L. Becker. “3D Printing of Poly(propylene fumarate) Oligomers: Evaluation of Resin Viscosity, Printing Characteristics and Mechanical Properties.” Biomacromolecules 20, no. 4 (April 2019): 1699–1708. https://doi.org/10.1021/acs.biomac.9b00076.
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  - Dilla, R. A., C. M. M. Motta, Y. Xu, Z. K. Zander, N. Bernard, C. G. Wiener, B. D. Vogt, and M. L. Becker. “Mechanically tunable, human mesenchymal stem cell viable poly(ethylene glycol)–oxime hydrogels with invariant precursor composition, concentration, and stoichiometry.” Materials Today Chemistry 11 (March 1, 2019): 244–52. https://doi.org/10.1016/j.mtchem.2018.11.003.
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  - Philip, Diana L., Elena A. Silantyeva, Matthew L. Becker, and Rebecca K. Willits. “RGD-Functionalized Nanofibers Increase Early GFAP Expression during Neural Differentiation of Mouse Embryonic Stem Cells.” Biomacromolecules 20, no. 3 (March 2019): 1443–54. https://doi.org/10.1021/acs.biomac.9b00018.
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  - Xia, X., Z. Qiang, G. Bass, M. L. Becker, and B. D. Vogt. “Morphological control of hydrothermally synthesized cobalt oxide particles using poly(vinyl pyrrolidone).” Colloid and Polymer Science 297, no. 1 (January 17, 2019): 59–67. https://doi.org/10.1007/s00396-018-4434-4.
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  - Cavanaugh, M., E. Silantyeva, G. P. Koh, E. Malekzadeh, W. D. Lanzinger, R. K. Willits, and M. L. Becker. “RGD-modified nanofibers enhance outcomes in rats after sciatic nerve injury.” Journal of Functional Biomaterials 10, no. 2 (January 1, 2019). https://doi.org/10.3390/jfb10020024.
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  - Guerra, Antonio J., Hernan Lara-Padilla, Matthew L. Becker, Ciro A. Rodriguez, and David Dean. “Photopolymerizable Resins for 3D-Printing Solid-Cured Tissue Engineered Implants.” Current Drug Targets 20, no. 8 (January 2019): 823–38. https://doi.org/10.2174/1389450120666190114122815.
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  - Dreger, Nathan Z., Zhaobo Fan, Zachary K. Zander, Chinnapatch Tantisuwanno, Molly C. Haines, Morgan Waggoner, Trenton Parsell, et al. “Amino acid-based Poly(ester urea) copolymer films for hernia-repair applications.” Biomaterials 182 (November 2018): 44–57. https://doi.org/10.1016/j.biomaterials.2018.08.003.
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  - Chen, K., N. Z. Dreger, F. Peng, B. D. Vogt, M. L. Becker, and M. Cakmak. “Nonlinear Mechano-Optical Behavior and Strain-Induced Structural Changes of l -Valine-Based Poly(ester urea)s.” Macromolecules 51, no. 20 (October 23, 2018): 8114–26. https://doi.org/10.1021/acs.macromol.8b01176.
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  - Dilla, R. A., C. M. M. Motta, S. R. Snyder, J. A. Wilson, C. Wesdemiotis, and M. L. Becker. “Synthesis and 3D Printing of PEG-Poly(propylene fumarate) Diblock and Triblock Copolymer Hydrogels.” Acs Macro Letters 7, no. 10 (October 16, 2018): 1254–60. https://doi.org/10.1021/acsmacrolett.8b00720.
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  - Chen, Yusheng, James A. Wilson, Shannon R. Petersen, Derek Luong, Sahar Sallam, Jialin Mao, Chrys Wesdemiotis, and Matthew L. Becker. “Ring-Opening Copolymerization of Maleic Anhydride with Functional Epoxides: Poly(propylene fumarate) Analogues Capable of Post-Polymerization Modification.” Angewandte Chemie (International Ed. in English) 57, no. 39 (September 2018): 12759–64. https://doi.org/10.1002/anie.201807419.
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  - Zander, Zachary K., Peiru Chen, Yen-Hao Hsu, Nathan Z. Dreger, Laura Savariau, Willie C. McRoy, Alec E. Cerchiari, Sean D. Chambers, Hazel A. Barton, and Matthew L. Becker. “Post-fabrication QAC-functionalized thermoplastic polyurethane for contact-killing catheter applications.” Biomaterials 178 (September 2018): 339–50. https://doi.org/10.1016/j.biomaterials.2018.05.010.
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  - Petersen, S. R., J. A. Wilson, and M. L. Becker. “Versatile Ring-Opening Copolymerization and Postprinting Functionalization of Lactone and Poly(propylene fumarate) Block Copolymers: Resorbable Building Blocks for Additive Manufacturing.” Macromolecules 51, no. 16 (August 28, 2018): 6202–8. https://doi.org/10.1021/acs.macromol.8b01372.
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  - Arno, Maria C., Ruairí P. Brannigan, Gina M. Policastro, Matthew L. Becker, and Andrew P. Dove. “pH-Responsive, Functionalizable Spyrocyclic Polycarbonate: A Versatile Platform for Biocompatible Nanoparticles.” Biomacromolecules 19, no. 8 (August 2018): 3427–34. https://doi.org/10.1021/acs.biomac.8b00744.
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  - Deming, Timothy J., Harm-Anton Klok, Steven P. Armes, Matthew L. Becker, Julie A. Champion, Eugene Y-X Chen, Sarah C. Heilshorn, et al. “Polymers at the Interface with Biology.” Biomacromolecules 19, no. 8 (August 2018): 3151–62. https://doi.org/10.1021/acs.biomac.8b01029.
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  - Childers, Erin P., Nathan Z. Dreger, Alex B. Ellenberger, Mary Beth Wandel, Karen Domino, Yanyi Xu, Derek Luong, et al. “Enhanced Rotator-Cuff Repair Using Platelet-Rich Plasma Adsorbed on Branched Poly(ester urea)s.” Biomacromolecules 19, no. 7 (July 2018): 3129–39. https://doi.org/10.1021/acs.biomac.8b00725.
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  - Silantyeva, Elena A., Wafaa Nasir, Jacqueline Carpenter, Olivia Manahan, Matthew L. Becker, and Rebecca K. Willits. “Accelerated neural differentiation of mouse embryonic stem cells on aligned GYIGSR-functionalized nanofibers.” Acta Biomaterialia 75 (July 2018): 129–39. https://doi.org/10.1016/j.actbio.2018.05.052.
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  - Dreger, N. Z., M. B. Wandel, L. L. Robinson, D. Luong, C. S. Søndergaard, M. Hiles, C. Premanandan, and M. L. Becker. “Preclinical in Vitro and in Vivo Assessment of Linear and Branched l -Valine-Based Poly(ester urea)s for Soft Tissue Applications.” Acs Biomaterials Science and Engineering 4, no. 4 (April 9, 2018): 1346–56. https://doi.org/10.1021/acsbiomaterials.7b00920.
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  - Li, Hang, Jukuan Zheng, Huifeng Wang, Mathew L. Becker, and Nic D. Leipzig. “Neural stem cell encapsulation and differentiation in strain promoted crosslinked polyethylene glycol-based hydrogels.” Journal of Biomaterials Applications 32, no. 9 (April 2018): 1222–30. https://doi.org/10.1177/0885328218755711.
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  - Wilson, James A., Derek Luong, Alex P. Kleinfehn, Sahar Sallam, Chrys Wesdemiotis, and Matthew L. Becker. “Magnesium Catalyzed Polymerization of End Functionalized Poly(propylene maleate) and Poly(propylene fumarate) for 3D Printing of Bioactive Scaffolds.” Journal of the American Chemical Society 140, no. 1 (January 2018): 277–84. https://doi.org/10.1021/jacs.7b09978.
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  - Zander, Zachary K., and Matthew L. Becker. “Antimicrobial and Antifouling Strategies for Polymeric Medical Devices.” Acs Macro Letters 7, no. 1 (January 2018): 16–25. https://doi.org/10.1021/acsmacrolett.7b00879.
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  - Sallam, Sahar, Yuanyuan Luo, Matthew L. Becker, and Chrys Wesdemiotis. “Multidimensional mass spectrometry characterization of isomeric biodegradable polyesters.” European Journal of Mass Spectrometry (Chichester, England) 23, no. 6 (December 2017): 402–10. https://doi.org/10.1177/1469066717711401.
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  - Yu, Jiayi, Yanyi Xu, Shan Li, Gabrielle V. Seifert, and Matthew L. Becker. “Three-Dimensional Printing of Nano Hydroxyapatite/Poly(ester urea) Composite Scaffolds with Enhanced Bioactivity.” Biomacromolecules 18, no. 12 (December 2017): 4171–83. https://doi.org/10.1021/acs.biomac.7b01222.
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  - Peterson, Gregory I., Andrey V. Dobrynin, and Matthew L. Becker. “Biodegradable Shape Memory Polymers in Medicine.” Advanced Healthcare Materials 6, no. 21 (November 2017). https://doi.org/10.1002/adhm.201700694.
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  - Li, Shan, Yanyi Xu, Jiayi Yu, and Matthew L. Becker. “Enhanced osteogenic activity of poly(ester urea) scaffolds using facile post-3D printing peptide functionalization strategies.” Biomaterials 141 (October 2017): 176–87. https://doi.org/10.1016/j.biomaterials.2017.06.038.
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  - Bhagat, Vrushali, and Matthew L. Becker. “Degradable Adhesives for Surgery and Tissue Engineering.” Biomacromolecules 18, no. 10 (October 2017): 3009–39. https://doi.org/10.1021/acs.biomac.7b00969.
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  - Xu, Yanyi, Derek Luong, Jason M. Walker, David Dean, and Matthew L. Becker. “Modification of Poly(propylene fumarate)-Bioglass Composites with Peptide Conjugates to Enhance Bioactivity.” Biomacromolecules 18, no. 10 (October 2017): 3168–77. https://doi.org/10.1021/acs.biomac.7b00828.
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  - Gao, Y., Y. Xu, A. Land, J. Harris, G. M. Policastro, E. P. Childers, T. Ritzman, J. Bundy, and M. L. Becker. “Sustained release of recombinant human growth hormone from bioresorbable poly(ester urea) nanofibers.” Acs Macro Letters 6, no. 8 (August 15, 2017): 875–80. https://doi.org/10.1021/acsmacrolett.7b00334.
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  - Peterson, G. I., E. P. Childers, H. Li, A. V. Dobrynin, and M. L. Becker. “Tunable Shape Memory Polymers from α-Amino Acid-Based Poly(ester urea)s.” Macromolecules 50, no. 11 (June 13, 2017): 4300–4308. https://doi.org/10.1021/acs.macromol.7b00680.
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  - Walker, J. M., E. Bodamer, A. Kleinfehn, Y. Luo, M. Becker, and D. Dean. “Design and mechanical characterization of solid and highly porous 3D printed poly(propylene fumarate) scaffolds.” Progress in Additive Manufacturing 2, no. 1–2 (June 1, 2017): 99–108. https://doi.org/10.1007/s40964-017-0021-3.
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  - Walker, Jason M., Emily Bodamer, Olivia Krebs, Yuanyuan Luo, Alex Kleinfehn, Matthew L. Becker, and David Dean. “Effect of Chemical and Physical Properties on the In Vitro Degradation of 3D Printed High Resolution Poly(propylene fumarate) Scaffolds.” Biomacromolecules 18, no. 4 (April 2017): 1419–25. https://doi.org/10.1021/acs.biomac.7b00146.
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  - Chen, K., J. Yu, G. Guzman, S. S. Es-Haghi, M. L. Becker, and M. Cakmak. “Role of Hydrogen Bonding on Nonlinear Mechano-Optical Behavior of l-Phenylalanine-Based Poly(ester urea)s.” Macromolecules 50, no. 3 (February 14, 2017): 1075–84. https://doi.org/10.1021/acs.macromol.6b02415.
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  - Vega, Sebastián L., Er Liu, Varun Arvind, Jared Bushman, Hak-Joon Sung, Matthew L. Becker, Sophie Lelièvre, Joachim Kohn, Pierre-Alexandre Vidi, and Prabhas V. Moghe. “High-content image informatics of the structural nuclear protein NuMA parses trajectories for stem/progenitor cell lineages and oncogenic transformation.” Experimental Cell Research 351, no. 1 (February 2017): 11–23. https://doi.org/10.1016/j.yexcr.2016.12.018.
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  - Alalwiat, Ahlam, Wen Tang, Selim Gerişlioğlu, Matthew L. Becker, and Chrys Wesdemiotis. “Mass Spectrometry and Ion Mobility Characterization of Bioactive Peptide-Synthetic Polymer Conjugates.” Analytical Chemistry 89, no. 2 (January 2017): 1170–77. https://doi.org/10.1021/acs.analchem.6b03553.
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  - Kim, Joseph J., Neal K. Bennett, Mitchel S. Devita, Sanjay Chahar, Satish Viswanath, Eunjee A. Lee, Giyoung Jung, et al. “Optical High Content Nanoscopy of Epigenetic Marks Decodes Phenotypic Divergence in Stem Cells.” Scientific Reports 7 (January 2017): 39406. https://doi.org/10.1038/srep39406.
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  - Xia, Y., Z. Qiang, B. Lee, M. L. Becker, and B. D. Vogt. “Solid state microwave synthesis of highly crystalline ordered mesoporous hausmannite Mn3O4 films.” Crystengcomm 19, no. 30 (January 1, 2017): 4294–4303. https://doi.org/10.1039/c7ce00900c.
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  - Zhou, J., V. Bhagat, and M. L. Becker. “Poly(ester urea)-Based Adhesives: Improved Deployment and Adhesion by Incorporation of Poly(propylene glycol) Segments.” Acs Applied Materials and Interfaces 8, no. 49 (December 14, 2016): 33423–29. https://doi.org/10.1021/acsami.6b09676.
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  - Peterson, G. I., A. V. Dobrynin, and M. L. Becker. “α-Amino Acid-Based Poly(Ester urea)s as Multishape Memory Polymers for Biomedical Applications.” Acs Macro Letters 5, no. 10 (October 18, 2016): 1176–79. https://doi.org/10.1021/acsmacrolett.6b00648.
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  - Bell, C. A., J. Yu, I. A. Barker, V. X. Truong, Z. Cao, A. V. Dobrinyin, M. L. Becker, and A. P. Dove. “Independent Control of Elastomer Properties through Stereocontrolled Synthesis.” Angewandte Chemie International Edition 55, no. 42 (October 10, 2016): 13076–80. https://doi.org/10.1002/anie.201606750.
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  - Childers, Erin P., Gregory I. Peterson, Alex B. Ellenberger, Karen Domino, Gabrielle V. Seifert, and Matthew L. Becker. “Adhesion of Blood Plasma Proteins and Platelet-rich Plasma on l-Valine-Based Poly(ester urea).” Biomacromolecules 17, no. 10 (October 2016): 3396–3403. https://doi.org/10.1021/acs.biomac.6b01195.
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  - Wade, Mary Beth, Eric Rodenberg, Umesh Patel, Bhavin Shah, and Matthew L. Becker. “Influence of Sterilization Technologies on Electrospun Poly(ester urea)s for Soft Tissue Repair.” Biomacromolecules 17, no. 10 (October 2016): 3363–74. https://doi.org/10.1021/acs.biomac.6b01158.
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  - Gao, Yaohua, Tai Yi, Toshiharu Shinoka, Yong Ung Lee, Darrell H. Reneker, Christopher K. Breuer, and Matthew L. Becker. “Pilot Mouse Study of 1 mm Inner Diameter (ID) Vascular Graft Using Electrospun Poly(ester urea) Nanofibers.” Advanced Healthcare Materials 5, no. 18 (September 2016): 2427–36. https://doi.org/10.1002/adhm.201600400.
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  - Castano, M., A. Alvarez, M. L. Becker, and J. E. Puskas. “Synthesis of polyisobutylene-polycaprolactone block copolymers using enzyme catalysis.” Express Polymer Letters 10, no. 8 (August 1, 2016): 693–700. https://doi.org/10.3144/expresspolymlett.2016.62.
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  - Qiang, Z., C. Ye, K. Lin, M. L. Becker, K. A. Cavicchi, and B. D. Vogt. “Evolution in surface morphology during rapid microwave annealing of PS-b-PMMA thin films.” Journal of Polymer Science, Part B: Polymer Physics 54, no. 15 (August 1, 2016): 1499–1506. https://doi.org/10.1002/polb.24043.
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  - Li, Xianfeng, N Sanjeeva Murthy, Matthew L. Becker, and Robert A. Latour. “Multiscale approach for the construction of equilibrated all-atom models of a poly(ethylene glycol)-based hydrogel.” Biointerphases 11, no. 2 (June 2016): 021002. https://doi.org/10.1116/1.4944829.
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  - Policastro, Gina M., and Matthew L. Becker. “Osteogenic growth peptide and its use as a bio-conjugate in regenerative medicine applications.” Wiley Interdisciplinary Reviews. Nanomedicine and Nanobiotechnology 8, no. 3 (May 2016): 449–64. https://doi.org/10.1002/wnan.1376.
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  - Ma, Yanrui, Gina M. Policastro, Qiyao Li, Jukuan Zheng, Robin Jacquet, William J. Landis, and Matthew L. Becker. “Concentration-Dependent hMSC Differentiation on Orthogonal Concentration Gradients of GRGDS and BMP-2 Peptides.” Biomacromolecules 17, no. 4 (April 2016): 1486–95. https://doi.org/10.1021/acs.biomac.6b00088.
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  - Zander, Z. K., F. Wang, M. L. Becker, and R. A. Weiss. “Ionomers for Tunable Softening of Thermoplastic Polyurethane.” Macromolecules 49, no. 3 (February 9, 2016): 926–34. https://doi.org/10.1021/acs.macromol.6b00005.
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  - Zander, Zachary K., Geng Hua, Clinton G. Wiener, Bryan D. Vogt, and Matthew L. Becker. “Control of Mesh Size and Modulus by Kinetically Dependent Cross-Linking in Hydrogels.” Advanced Materials (Deerfield Beach, Fla.) 27, no. 40 (October 2015): 6283–88. https://doi.org/10.1002/adma.201501822.
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  - Gao, Y., E. P. Childers, and M. L. Becker. “L -Leucine-Based Poly(ester urea)s for Vascular Tissue Engineering.” Acs Biomaterials Science and Engineering 1, no. 9 (September 14, 2015): 795–804. https://doi.org/10.1021/acsbiomaterials.5b00168.
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  - Liu, K., Y. M. Chen, G. M. Policastro, M. L. Becker, and Y. Zhu. “Three-Dimensional Bicontinuous Graphene Monolith from Polymer Templates.” Acs Nano 9, no. 6 (June 23, 2015): 6041–49. https://doi.org/10.1021/acsnano.5b01006.
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  - Yu, J., F. Lin, and M. L. Becker. “Branched amino acid based poly(ester urea)s with tunable thermal and water uptake properties.” Macromolecules 48, no. 9 (May 12, 2015): 2916–24. https://doi.org/10.1021/acs.macromol.5b00376.
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  - Zhou, J., K. Mishra, V. Bhagat, A. Joy, and M. L. Becker. “Thermoresponsive dual emission nanosensor based on quantum dots and dye labeled poly(N-isopropylacrylamide).” Polymer Chemistry 6, no. 15 (April 21, 2015): 2813–16. https://doi.org/10.1039/c4py01781a.
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  - Policastro, Gina M., Fei Lin, Laura A. Smith Callahan, Andrew Esterle, Matthew Graham, Kimberly Sloan Stakleff, and Matthew L. Becker. “OGP functionalized phenylalanine-based poly(ester urea) for enhancing osteoinductive potential of human mesenchymal stem cells.” Biomacromolecules 16, no. 4 (April 2015): 1358–71. https://doi.org/10.1021/acs.biomac.5b00153.
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  - Defante, Adrian P., Tarak N. Burai, Matthew L. Becker, and Ali Dhinojwala. “Consequences of water between two hydrophobic surfaces on adhesion and wetting.” Langmuir : The Acs Journal of Surfaces and Colloids 31, no. 8 (March 2015): 2398–2406. https://doi.org/10.1021/la504564w.
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  - Zhang, Yuanzhong, Sarang M. Bhaway, Yi Wang, Kevin A. Cavicchi, Matthew L. Becker, and Bryan D. Vogt. “Rapid (<3 min) microwave synthesis of block copolymer templated ordered mesoporous metal oxide and carbonate films using nitrate-citric acid systems.” Chemical Communications (Cambridge, England) 51, no. 24 (March 2015): 4997–5000. https://doi.org/10.1039/c4cc09808k.
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  - Castano, M., K. S. Seo, K. Guo, M. L. Becker, C. Wesdemiotis, and J. E. Puskas. “Green polymer chemistry: Synthesis of symmetric and asymmetric telechelic ethylene glycol oligomers.” Polymer Chemistry 6, no. 7 (February 21, 2015): 1137–42. https://doi.org/10.1039/c4py01223b.
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  - Zheng, J., G. Hua, J. Yu, F. Lin, M. B. Wade, D. H. Reneker, and M. L. Becker. “Post-electrospinning "triclick" functionalization of degradable polymer nanofibers.” Acs Macro Letters 4, no. 2 (February 17, 2015): 207–13. https://doi.org/10.1021/mz500759n.
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  - Li, Shan, Jiayi Yu, Mary Beth Wade, Gina M. Policastro, and Matthew L. Becker. “Radiopaque, iodine functionalized, phenylalanine-based poly(ester urea)s.” Biomacromolecules 16, no. 2 (February 2015): 615–24. https://doi.org/10.1021/bm501669u.
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  - Zheng, Jukuan, Dimitria Kontoveros, Fei Lin, Geng Hua, Darrell H. Reneker, Matthew L. Becker, and Rebecca K. Willits. “Enhanced Schwann cell attachment and alignment using one-pot "dual click" GRGDS and YIGSR derivatized nanofibers.” Biomacromolecules 16, no. 1 (January 2015): 357–63. https://doi.org/10.1021/bm501552t.
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  - Zheng, J., Y. Chen, A. Karim, and M. L. Becker. “Dopamine-based copper-free click kit for efficient surface functionalization.” Acs Macro Letters 3, no. 10 (October 21, 2014): 1084–87. https://doi.org/10.1021/mz5005162.
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  - Castano, M., M. L. Becker, and J. E. Puskas. “New method for the synthesis of fully aliphatic telechelic α,ω-dihydroxy-polyisobutylene.” Polymer Chemistry 5, no. 18 (September 21, 2014): 5436–42. https://doi.org/10.1039/c4py00569d.
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  - Castano, M., J. Zheng, J. E. Puskas, and M. L. Becker. “Enzyme-catalyzed ring-opening polymerization of ε-caprolactone using alkyne functionalized initiators.” Polymer Chemistry 5, no. 6 (March 21, 2014): 1891–96. https://doi.org/10.1039/c3py01536j.
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  - Yu, J., F. Lin, P. Lin, Y. Gao, and M. L. Becker. “Phenylalanine-based poly(ester urea): Synthesis, characterization, and in vitro degradation.” Macromolecules 47, no. 1 (January 14, 2014): 121–29. https://doi.org/10.1021/ma401752b.
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  - Seo, K. S., M. Castano, M. Casiano, C. Wesdemiotis, M. L. Becker, and J. E. Puskas. “Enzyme-catalyzed quantitative chain-end functionalization of poly(ethylene glycol)s under solventless conditions.” Rsc Advances 4, no. 4 (January 1, 2014): 1683–88. https://doi.org/10.1039/c3ra46070c.
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  - Lin, F., J. Yu, W. Tang, J. Zheng, S. Xie, and M. L. Becker. “Postelectrospinning "click" modification of degradable amino acid-based poly(ester urea) nanofibers.” Macromolecules 46, no. 24 (December 23, 2013): 9515–25. https://doi.org/10.1021/ma401964e.
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  - Liu, X., J. Zhou, J. Zheng, M. L. Becker, and X. Gong. “Water-soluble CdTe quantum dots as an anode interlayer for solution-processed near infrared polymer photodetectors.” Nanoscale 5, no. 24 (December 2, 2013): 12474–79. https://doi.org/10.1039/c3nr03602b.
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  - Callahan, Laura A Smith, Sibai Xie, Ian A. Barker, Jukuan Zheng, Darrell H. Reneker, Andrew P. Dove, and Matthew L. Becker. “Directed differentiation and neurite extension of mouse embryonic stem cell on aligned poly(lactide) nanofibers functionalized with YIGSR peptide.” Biomaterials 34, no. 36 (December 2013): 9089–95. https://doi.org/10.1016/j.biomaterials.2013.08.028.
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  - Li, Y., Z. Wang, J. Zheng, H. Su, F. Lin, K. Guo, X. Feng, et al. “Cascading one-pot synthesis of single-tailed and asymmetric multitailed giant surfactants.” Acs Macro Letters 2, no. 11 (November 19, 2013): 1026–32. https://doi.org/10.1021/mz400519c.
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  - Lin, Fei, Jiayi Yu, Wen Tang, Jukuan Zheng, Adrian Defante, Kai Guo, Chrys Wesdemiotis, and Matthew L. Becker. “Peptide-functionalized oxime hydrogels with tunable mechanical properties and gelation behavior.” Biomacromolecules 14, no. 10 (October 2013): 3749–58. https://doi.org/10.1021/bm401133r.
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  - Castano, Marcela, Kwang Su Seo, Eun Hye Kim, Matthew L. Becker, and Judit E. Puskas. “Green polymer chemistry VIII: synthesis of halo-ester-functionalized poly(ethylene glycol)s via enzymatic catalysis.” Macromolecular Rapid Communications 34, no. 17 (September 2013): 1375–80. https://doi.org/10.1002/marc.201300430.
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  - Smith Callahan, Laura A., Gina M. Policastro, Sharon L. Bernard, Erin P. Childers, Ronna Boettcher, and Matthew L. Becker. “Influence of discrete and continuous culture conditions on human mesenchymal stem cell lineage choice in RGD concentration gradient hydrogels.” Biomacromolecules 14, no. 9 (September 2013): 3047–54. https://doi.org/10.1021/bm4006112.
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  - Tang, Wen, Yanrui Ma, Sibai Xie, Kai Guo, Bryan Katzenmeyer, Chrys Wesdemiotis, and Matthew L. Becker. “Valency-dependent affinity of bioactive hydroxyapatite-binding dendrons.” Biomacromolecules 14, no. 9 (September 2013): 3304–13. https://doi.org/10.1021/bm400908c.
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  - Su, H., J. Zheng, Z. Wang, F. Lin, X. Feng, X. H. Dong, M. L. Becker, S. Z. D. Cheng, W. B. Zhang, and Y. Li. “Sequential triple "click" approach toward polyhedral oligomeric silsesquioxane-based multiheaded and multitailed giant surfactants.” Acs Macro Letters 2, no. 8 (August 20, 2013): 645–50. https://doi.org/10.1021/mz4002723.
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  - Lin, Fei, Jukuan Zheng, Jiayi Yu, Jinjun Zhou, and Matthew L. Becker. “Cascading "Triclick" functionalization of poly(caprolactone) thin films quantified via a quartz crystal microbalance.” Biomacromolecules 14, no. 8 (August 2013): 2857–65. https://doi.org/10.1021/bm400711q.
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  - Smith Callahan, Laura A., Erin P. Childers, Sharon L. Bernard, Scott D. Weiner, and Matthew L. Becker. “Maximizing phenotype constraint and extracellular matrix production in primary human chondrocytes using arginine-glycine-aspartate concentration gradient hydrogels.” Acta Biomaterialia 9, no. 7 (July 2013): 7420–28. https://doi.org/10.1016/j.actbio.2013.04.005.
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  - Bandyopadhyay, D., G. Singh, M. L. Becker, and A. Karim. “Capillary wave confinement-induced stabilization of polymer films.” Acs Applied Materials and Interfaces 5, no. 10 (May 22, 2013): 4006–10. https://doi.org/10.1021/am4002502.
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  - Zhou, J., S. Xie, E. F. Amond, and M. L. Becker. “Tuning energy levels of low bandgap semi-random two acceptor copolymers.” Macromolecules 46, no. 9 (May 14, 2013): 3391–94. https://doi.org/10.1021/ma400531v.
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  - Smith Callahan, L. A., Y. Ma, C. M. Stafford, and M. L. Becker. “Concentration dependent neural differentiation and neurite extension of mouse ESC on primary amine-derivatized surfaces.” Biomaterials Science 1, no. 5 (May 1, 2013): 537–44. https://doi.org/10.1039/c3bm00161j.
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  - Zheng, J., S. Xie, F. Lin, G. Hua, T. Yu, D. H. Reneker, and M. L. Becker. “4-Dibenzocyclooctynol (DIBO) as an initiator for poly(ε-caprolactone): Copper-free clickable polymer and nanofiber-based scaffolds.” Polymer Chemistry 4, no. 7 (April 7, 2013): 2215–18. https://doi.org/10.1039/c3py00153a.
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  - Callahan, Laura A Smith, Anna M. Ganios, Erin P. Childers, Scott D. Weiner, and Matthew L. Becker. “Primary human chondrocyte extracellular matrix formation and phenotype maintenance using RGD-derivatized PEGDM hydrogels possessing a continuous Young's modulus gradient.” Acta Biomaterialia 9, no. 4 (April 2013): 6095–6104. https://doi.org/10.1016/j.actbio.2012.12.028.
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  - Ma, Yanrui, Jukuan Zheng, Emily F. Amond, Christopher M. Stafford, and Matthew L. Becker. “Facile fabrication of "dual click" one- and two-dimensional orthogonal peptide concentration gradients.” Biomacromolecules 14, no. 3 (March 2013): 665–71. https://doi.org/10.1021/bm301731h.
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  - Stakleff, Kimberly Sloan, Fei Lin, Laura A. Smith Callahan, Mary Beth Wade, Andrew Esterle, James Miller, Matthew Graham, and Matthew L. Becker. “Resorbable, amino acid-based poly(ester urea)s crosslinked with osteogenic growth peptide with enhanced mechanical properties and bioactivity.” Acta Biomaterialia 9, no. 2 (February 2013): 5132–42. https://doi.org/10.1016/j.actbio.2012.08.035.
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  - Rao, T., G. Singh, S. Xie, A. Karim, and M. L. Becker. “2-D gold nanoparticle arrays from thermally directed self-assembly of peptide-derivatized block copolymers.” Soft Matter 9, no. 33 (January 1, 2013): 8023–32. https://doi.org/10.1039/c3sm51106e.
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  - Vega, Sebastián L., Er Liu, Parth J. Patel, Anthony B. Kulesa, Aaron L. Carlson, Yanrui Ma, Matthew L. Becker, and Prabhas V. Moghe. “High-content imaging-based screening of microenvironment-induced changes to stem cells.” Journal of Biomolecular Screening 17, no. 9 (October 2012): 1151–62. https://doi.org/10.1177/1087057112453853.
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  - Zheng, Jukuan, Kaiyi Liu, Darrell H. Reneker, and Matthew L. Becker. “Post-assembly derivatization of electrospun nanofibers via strain-promoted azide alkyne cycloaddition.” Journal of the American Chemical Society 134, no. 41 (October 2012): 17274–77. https://doi.org/10.1021/ja307647x.
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  - Zartman, G. D., S. Cheng, X. Li, F. Lin, M. L. Becker, and S. Q. Wang. “How melt-stretching affects mechanical behavior of polymer glasses.” Macromolecules 45, no. 16 (August 28, 2012): 6719–32. https://doi.org/10.1021/ma300955h.
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  - Zheng, J., L. A. Smith Callahan, J. Hao, K. Guo, C. Wesdemiotis, R. A. Weiss, and M. L. Becker. “Strain-promoted cross-linking of PEG-based hydrogels via copper- free cycloaddition.” Acs Macro Letters 1, no. 8 (August 21, 2012): 1071–73. https://doi.org/10.1021/mz3003775.
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  - Callahan, Laura A Smith, Anna M. Ganios, Denise L. McBurney, Matthew F. Dilisio, Scott D. Weiner, Walter E. Horton, and Matthew L. Becker. “ECM production of primary human and bovine chondrocytes in hybrid PEG hydrogels containing type I collagen and hyaluronic acid.” Biomacromolecules 13, no. 5 (May 2012): 1625–31. https://doi.org/10.1021/bm3003336.
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  - Rao, T., X. H. Dong, B. C. Katzenmeyer, C. Wesdemiotis, S. Z. D. Cheng, and M. L. Becker. “High-fidelity fabrication of Au-polymer Janus nanoparticles using a solution template approach.” Soft Matter 8, no. 10 (March 14, 2012): 2965–71. https://doi.org/10.1039/c2sm07002b.
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  - Yu, Jing, Matthew L. Becker, and Gustavo A. Carri. “The influence of amino acid sequence and functionality on the binding process of peptides onto gold surfaces.” Langmuir : The Acs Journal of Surfaces and Colloids 28, no. 2 (January 2012): 1408–17. https://doi.org/10.1021/la204109r.
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  - Moore, Nicole M., Nancy J. Lin, Nathan D. Gallant, and Matthew L. Becker. “Synergistic enhancement of human bone marrow stromal cell proliferation and osteogenic differentiation on BMP-2-derived and RGD peptide concentration gradients.” Acta Biomaterialia 7, no. 5 (May 2011): 2091–2100. https://doi.org/10.1016/j.actbio.2011.01.019.
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  - Fagan, Jeffrey A., Barry J. Bauer, Erik K. Hobbie, Matthew L. Becker, Angela R. Hight Walker, Jeffrey R. Simpson, Jaehun Chun, et al. “Carbon nanotubes: measuring dispersion and length.” Advanced Materials (Deerfield Beach, Fla.) 23, no. 3 (January 2011): 338–48. https://doi.org/10.1002/adma.201001756.
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  - Acharya, Abhinav P., Natalia V. Dolgova, Nicole M. Moore, Chang-Qing Xia, Michael J. Clare-Salzler, Matthew L. Becker, Nathan D. Gallant, and Benjamin G. Keselowsky. “The modulation of dendritic cell integrin binding and activation by RGD-peptide density gradient substrates.” Biomaterials 31, no. 29 (October 2010): 7444–54. https://doi.org/10.1016/j.biomaterials.2010.06.025.
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  - Yu, Jing, Matthew L. Becker, and Gustavo A. Carri. “A molecular dynamics simulation of the stability-limited growth mechanism of peptide-mediated gold-nanoparticle synthesis.” Small (Weinheim an Der Bergstrasse, Germany) 6, no. 20 (October 2010): 2242–45. https://doi.org/10.1002/smll.201000889.
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  - Park, Jung Jin, Michael C. Weiger, Silvia H De Paoli Lacerda, Denis Pristinski, Matthew L. Becker, Jack F. Douglas, Dharmaraj Raghavan, and Alamgir Karim. “Characterization of non-equilibrium nanoparticle adsorption on a model biological substrate.” Langmuir : The Acs Journal of Surfaces and Colloids 26, no. 7 (April 2010): 4822–30. https://doi.org/10.1021/la903581w.
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  - Weiger, Michael C., Jung Jin Park, Marc D. Roy, Christopher M. Stafford, Alamgir Karim, and Matthew L. Becker. “Quantification of the binding affinity of a specific hydroxyapatite binding peptide.” Biomaterials 31, no. 11 (April 2010): 2955–63. https://doi.org/10.1016/j.biomaterials.2010.01.012.
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  - Moore, Nicole M., Nancy J. Lin, Nathan D. Gallant, and Matthew L. Becker. “The use of immobilized osteogenic growth peptide on gradient substrates synthesized via click chemistry to enhance MC3T3-E1 osteoblast proliferation.” Biomaterials 31, no. 7 (March 2010): 1604–11. https://doi.org/10.1016/j.biomaterials.2009.11.011.
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  - Bailey, M. M., C. M. Mahoney, K. E. Dempah, J. M. Davis, M. L. Becker, S. Khondee, E. J. Munson, and C. Berkland. “Fluorinated copolymer nanoparticles for multimodal imaging applications.” Macromolecular Rapid Communications 31, no. 1 (January 4, 2010): 87–92. https://doi.org/10.1002/marc.200900505.
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  - Lacerda, Silvia H De Paoli, Jung Jin Park, Curt Meuse, Denis Pristinski, Matthew L. Becker, Alamgir Karim, and Jack F. Douglas. “Interaction of gold nanoparticles with common human blood proteins.” Acs Nano 4, no. 1 (January 2010): 365–79. https://doi.org/10.1021/nn9011187.
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  - Simpson, J. R., J. A. Fagan, M. L. Becker, E. K. Hobbie, and A. R. Hight Walker. “The effect of dispersant on defects in length-separated single-wall carbon nanotubes measured by Raman spectroscopy.” Carbon 47, no. 14 (November 1, 2009): 3238–41. https://doi.org/10.1016/j.carbon.2009.07.037.
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  - Jakupciak, J. P., N. D. Gallant, A. H. Smith, M. L. Becker, A. Tona, and D. H. Atha. “Improved methods and standards for telomerase detection: quantitative histopathology using antibody staining.” Biotechnic & Histochemistry : Official Publication of the Biological Stain Commission 84, no. 5 (October 2009): 195–206. https://doi.org/10.3109/10520290903039060.
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  - Aamer, Khaled A., Kirsten L. Genson, Joachim Kohn, and Matthew L. Becker. “Impact of polymer-bound iodine on fibronectin adsorption and osteoblast cell morphology in radiopaque medical polymers: tyrosine-derived polycarbonate blends as a model system.” Biomacromolecules 10, no. 9 (September 2009): 2418–26. https://doi.org/10.1021/bm900327b.
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  - Stanley, Scott K., Matthew L. Becker, Eric K. Lin, and Wen-li Wu. “Inhibitory effects of a phage-derived peptide on Au nanocrystal nucleation and growth.” Langmuir : The Acs Journal of Surfaces and Colloids 25, no. 18 (September 2009): 10886–92. https://doi.org/10.1021/la901222k.
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  - Liu, Er, Matthew D. Treiser, Hiral Patel, Hak-Joon Sung, Kristen E. Roskov, Joachim Kohn, Matthew L. Becker, and Prabhas V. Moghe. “High-content profiling of cell responsiveness to graded substrates based on combinyatorially variant polymers.” Combinatorial Chemistry & High Throughput Screening 12, no. 7 (August 2009): 646–55. https://doi.org/10.2174/138620709788923737.
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  - Aamer, K. A., C. M. Stafford, L. J. Richter, J. Kohn, and M. L. Becker. “Thin film elastic modulus of degradable tyrosine-derived polycarbonate biomaterials and their blends.” Macromolecules 42, no. 4 (February 24, 2009): 1212–18. https://doi.org/10.1021/ma802115b.
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  - Hobbie, Erik K., Jeffrey A. Fagan, Matthew L. Becker, Steven D. Hudson, Nikta Fakhri, and Matteo Pasquali. “Self-assembly of ordered nanowires in biological suspensions of single-wall carbon nanotubes.” Acs Nano 3, no. 1 (January 2009): 189–96. https://doi.org/10.1021/nn800609y.
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  - Fagan, J. A., M. L. Becker, J. Chun, P. Nie, B. J. Bauer, J. R. Simpson, A. Hight-Walker, and E. K. Hobbie. “Centrifugal length separation of carbon nanotubes.” Langmuir 24, no. 24 (December 16, 2008): 13880–89. https://doi.org/10.1021/la801388a.
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  - Yang, Y., D. Bolikal, M. L. Becker, J. Kohn, D. N. Zeiger, and C. G. Simon. “Combinatorial polymer scaffold libraries for screening cell-biomaterial interactions in 3D.” Advanced Materials 20, no. 11 (June 4, 2008): 2037–43. https://doi.org/10.1002/adma.200702088.
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  - Morgan, Abby W., Kristen E. Roskov, Sheng Lin-Gibson, David L. Kaplan, Matthew L. Becker, and Carl G. Simon. “Characterization and optimization of RGD-containing silk blends to support osteoblastic differentiation.” Biomaterials 29, no. 16 (June 2008): 2556–63. https://doi.org/10.1016/j.biomaterials.2008.02.007.
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  - Roy, M. D., S. K. Stanley, E. J. Amis, and M. L. Becker. “Identification of a highly specific hydroxyapatite-binding peptide using phage display.” Advanced Materials 20, no. 10 (May 19, 2008): 1830–36. https://doi.org/10.1002/adma.200702322.
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  - Haggenmueller, Reto, Sameer S. Rahatekar, Jeffrey A. Fagan, Jaehun Chun, Matthew L. Becker, Rajesh R. Naik, Todd Krauss, et al. “Comparison of the quality of aqueous dispersions of single wall carbon nanotubes using surfactants and biomolecules.” Langmuir : The Acs Journal of Surfaces and Colloids 24, no. 9 (May 2008): 5070–78. https://doi.org/10.1021/la703008r.
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  - Roy, Marc D., Andrew A. Herzing, Silvia H. De Paoli Lacerda, and Matthew L. Becker. “Emission-tunable microwave synthesis of highly luminescent water soluble CdSe/ZnS quantum dots.” Chemical Communications (Cambridge, England), no. 18 (May 2008): 2106–8. https://doi.org/10.1039/b800060c.
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  - Yang, Yanyin, Shauna M. Dorsey, Matthew L. Becker, Sheng Lin-Gibson, Gary E. Schumacher, Glenn M. Flaim, Joachim Kohn, and Carl G. Simon. “X-ray imaging optimization of 3D tissue engineering scaffolds via combinatorial fabrication methods.” Biomaterials 29, no. 12 (April 2008): 1901–11. https://doi.org/10.1016/j.biomaterials.2007.12.042.
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  - Bauer, B. J., M. L. Becker, V. Bajpai, J. A. Fagan, E. K. Hobbie, K. Migler, C. M. Guttman, and W. R. Blair. “Measurement of single-wall nanotube dispersion by size exclusion chromatography.” Journal of Physical Chemistry C 111, no. 48 (December 6, 2007): 17914–18. https://doi.org/10.1021/jp071494q.
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  - De Paoli Lacerda, S. H., J. F. Douglas, S. D. Hudson, M. Roy, J. M. Johnson, M. L. Becker, and A. Karim. “Quantum Mazes: Luminescent Labyrinthine Semiconductor Nanocrystals Having a Narrow Emission Spectrum.” Acs Nano 1, no. 4 (November 1, 2007): 337–47. https://doi.org/10.1021/nn700111c.
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  - Fagan, J. A., J. R. Simpson, B. J. Bauer, S. H. D. P. Lacerda, M. L. Becker, J. Chun, K. B. Migler, A. R. H. Walker, and E. K. Hobbie. “Length-dependent optical effects in single-wall carbon nanotubes.” Journal of the American Chemical Society 129, no. 34 (August 29, 2007): 10607–12. https://doi.org/10.1021/ja073115c.
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  - Simon, Carl G., Jean S. Stephens, Shauna M. Dorsey, and Matthew L. Becker. “Fabrication of combinatorial polymer scaffold libraries.” The Review of Scientific Instruments 78, no. 7 (July 2007): 072207. https://doi.org/10.1063/1.2755761.
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  - Becker, M. L., J. A. Fagan, N. D. Gallant, B. J. Bauer, V. Bajpai, E. K. Hobbie, S. H. Lacerda, K. B. Migler, and J. P. Jakupciak. “Length-dependent uptake of DNA-wrapped single-walled carbon nanotubes.” Advanced Materials 19, no. 7 (April 6, 2007): 939–45. https://doi.org/10.1002/adma.200602667.
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  - Gallant, N. D., K. A. Lavery, E. J. Amis, and M. L. Becker. “Universal gradient substrates for "click" biofunctionalization.” Advanced Materials 19, no. 7 (April 6, 2007): 965–69. https://doi.org/10.1002/adma.200602221.
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  - Lin, Nancy J., LeeAnn O. Bailey, Matthew L. Becker, Newell R. Washburn, and Lori A. Henderson. “Macrophage response to methacrylate conversion using a gradient approach.” Acta Biomaterialia 3, no. 2 (March 2007): 163–73. https://doi.org/10.1016/j.actbio.2006.10.001.
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  - Bauer, B. J., E. K. Hobbie, and M. L. Becker. “Small-angle neutron scattering from labeled single-wall carbon nanotubes.” Macromolecules 39, no. 7 (April 4, 2006): 2637–42. https://doi.org/10.1021/ma0527303.
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  - Bailey, LeeAnn O., Matthew L. Becker, Jean S. Stephens, Nathan D. Gallant, Christine M. Mahoney, Newell R. Washburn, Aarti Rege, Joachim Kohn, and Eric J. Amis. “Cellular response to phase-separated blends of tyrosine-derived polycarbonates.” Journal of Biomedical Materials Research. Part A 76, no. 3 (March 2006): 491–502. https://doi.org/10.1002/jbm.a.30527.
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  - Fry, D., B. Langhorst, H. Wang, M. L. Becker, B. J. Bauer, E. A. Grulke, and E. K. Hobbie. “Rheo-optical studies of carbon nanotube suspensions.” Journal of Chemical Physics 124, no. 5 (February 13, 2006). https://doi.org/10.1063/1.2159488.
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  - Hobbie, E. K., B. J. Bauer, J. Stephens, M. L. Becker, P. McGuiggan, S. D. Hudson, and H. Wang. “Colloidal particles coated and stabilized by DNA-wrapped carbon nanotubes.” Langmuir : The Acs Journal of Surfaces and Colloids 21, no. 23 (November 2005): 10284–87. https://doi.org/10.1021/la051827f.
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  - Sun, Xiankai, Raffaella Rossin, Jeffrey L. Turner, Matthew L. Becker, Maisie J. Joralemon, Michael J. Welch, and Karen L. Wooley. “An assessment of the effects of shell cross-linked nanoparticle size, core composition, and surface PEGylation on in vivo biodistribution.” Biomacromolecules 6, no. 5 (September 2005): 2541–54. https://doi.org/10.1021/bm050260e.
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  - Turner, J. L., M. L. Becker, X. Li, J. S. A. Taylor, and K. L. Wooley. “PNA-directed solution- And surface-assembly of shell crosslinked (SCK) nanoparticle conjugates.” Journal of Materials Chemistry 15, no. 22 (June 14, 2005): 69–78. https://doi.org/10.1039/b417653g.
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  - Hammouda, B., F. Horkay, and M. L. Becker. “Clustering and solvation in poly(acrylic acid) polyelectrolyte solutions.” Macromolecules 38, no. 5 (March 8, 2005): 2019–21. https://doi.org/10.1021/ma047960g.
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  - Becker, Matthew L., Jianquan Liu, and Karen L. Wooley. “Functionalized micellar assemblies prepared via block copolymers synthesized by living free radical polymerization upon peptide-loaded resins.” Biomacromolecules 6, no. 1 (January 2005): 220–28. https://doi.org/10.1021/bm049551y.
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  - Becker, Matthew L., Edward E. Remsen, Dipanjan Pan, and Karen L. Wooley. “Peptide-derivatized shell-cross-linked nanoparticles. 1. Synthesis and characterization.” Bioconjugate Chemistry 15, no. 4 (July 2004): 699–709. https://doi.org/10.1021/bc049946e.
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  - Becker, Matthew L., LeeAnn O. Bailey, and Karen L. Wooley. “Peptide-derivatized shell-cross-linked nanoparticles. 2. Biocompatibility evaluation.” Bioconjugate Chemistry 15, no. 4 (July 2004): 710–17. https://doi.org/10.1021/bc049945m.
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  - Joralemon, Maisie J., K Shanmugananda Murthy, Edward E. Remsen, Matthew L. Becker, and Karen L. Wooley. “Synthesis, characterization, and bioavailability of mannosylated shell cross-linked nanoparticles.” Biomacromolecules 5, no. 3 (May 2004): 903–13. https://doi.org/10.1021/bm0344710.
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  - Becker, M. L., J. Liu, and K. L. Wooley. “Erratum: Peptide-polymer bioconjugates: Hybrid block copolymers generated via living radical polymerizations from resin-supported peptides (Chemical Communications 2003 (180)).” Chemical Communications, no. 6 (March 21, 2003): 802.
  - Becker, Matthew L., Jianquan Liu, and Karen L. Wooley. “Peptide-polymer bioconjugates: hybrid block copolymers generated via living radical polymerizations from resin-supported peptides.” Chemical Communications (Cambridge, England), no. 2 (January 2003): 180–81. https://doi.org/10.1039/b209557b.
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  - Becker, M. L., E. E. Remsen, and K. L. Wooley. “Diblock copolymers, micelles, and shell-crosslinked nanoparticles containing poly(4-fluorostyrene): Tools for detailed analyses of nanostructured materials.” Journal of Polymer Science, Part A: Polymer Chemistry 39, no. 23 (December 1, 2001): 4152–66. https://doi.org/10.1002/pola.10070.
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- Book Sections
  - Moore, N. M., and M. L. Becker. “Bioactive Self-Assembled Monolayer Gradients.” In Soft Matter Gradient Surfaces: Methods and Applications, 329–63, 2012. https://doi.org/10.1002/9781118166086.ch13.
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- Conference Papers
  - Weiger, M. C., K. Aamer, J. Kohn, and M. L. Becker. “Advancing SPRi measurements with novel biosensors for studying surface-biomolecule interactions.” In Acs Symposium Series, 1054:109–24, 2010. https://doi.org/10.1021/bk-2010-1054.ch005.
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  - Becker, M. L., M. D. Roy, S. K. Stanley, and E. J. Amis. “Identification of a highly-specific hydroxyapatite-binding peptide using phage display.” In 8th World Biomaterials Congress 2008, 4:1903, 2008.
  - Gallant, N. D., E. J. Amis, and M. L. Becker. “Bioactive surface gradients for combinatorial studies of cell adhesion.” In 8th World Biomaterials Congress 2008, 2:744, 2008.
  - Bauer, B. J., V. Bajpai, J. A. Fagan, M. L. Becker, and E. K. Hobbie. “Chromatographic separation of single wall carbon nanotubes.” In Materials Research Society Symposium Proceedings, 922:82–88, 2006. https://doi.org/10.1557/proc-0922-u09-01.
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  - Becker, M. L., M. J. Joralemon, E. E. Remsen, P. J. Endres, L. Cegelski, H. Huang, J. Schaefer, and K. L. Wooley. “Biocompatible surface functionalized shell crosslinked nanoparticles for use in biological applications.” In American Chemical Society, Polymer Preprints, Division of Polymer Chemistry, 43:682–83, 2002.
  - Becker, M. L., M. J. Joralemon, J. Liu, Q. Ma, K. S. Murthy, K. Qi, E. E. Remsen, Q. Zhang, and K. L. Wooley. “Synthetic methodologies for the surface derivatization of shell crosslinked nanoparticles.” In American Chemical Society, Polymer Preprints, Division of Polymer Chemistry, 43:323, 2002.
  - Becker, M. L., and K. L. Wooley. “Radical-based preparation of block copolymers containing fluorine tags: tools for detailed analysis of nanostructured materials.” In American Chemical Society, Polymer Preprints, Division of Polymer Chemistry, 41:1328–29, 2000.
Teaching & Mentoring
Recent Courses
- CHEM 393: Research Independent Study 2022
- CHEM 394: Research Independent Study 2022
- CHEM 493: Research Independent Study 2022
- CHEM 494: Research Independent Study 2022
- CHEM 590: Special Topics in Chemistry 2022
- ME 490: Special Topics in Mechanical Engineering 2022
- ME 555: Advanced Topics in Mechanical Engineering 2022
- MSEG 591: Independent Study 2022
- CHEM 110DL: Honors Chemistry: Core Concepts in Context 2021
- CHEM 393: Research Independent Study 2021
- CHEM 394: Research Independent Study 2021
- CHEM 493: Research Independent Study 2021
- CHEM 494: Research Independent Study 2021
- CHEM 590: Special Topics in Chemistry 2021
- CHEM 110DL: Honors Chemistry: Core Concepts in Context 2020
- CHEM 393: Research Independent Study 2020
- CHEM 394: Research Independent Study 2020
- CHEM 493: Research Independent Study 2020
- CHEM 494: Research Independent Study 2020
- CHEM 590: Special Topics in Chemistry 2020

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