Rapid phase-cycled two-dimensional optical spectroscopy in fluorescence and transmission mode

Journal Article (Journal Article)

Two dimensional magnetic and optical spectra contain information about structure and dynamics inaccessible to the linear spectroscopist. Recently, phase cycling techniques in optical spectroscopy have extended the capabilities of two-dimensional electronic spectroscopy. Here, we present a method to generate collinear pump/probe pulses at high update rates for two-dimensional electronic spectroscopy. Both fluorescence mode and transmission mode photon echo data from rubidium vapor is presented. © 2005 Optical Society of America.

Full Text

Duke Authors

Cited Authors

  • Wagner, W; Li, C; Semmlow, J; Warren, WS

Published Date

  • May 15, 2005

Published In

Volume / Issue

  • 13 / 10

Start / End Page

  • 3697 - 3706

Electronic International Standard Serial Number (EISSN)

  • 1094-4087

International Standard Serial Number (ISSN)

  • 1094-4087

Digital Object Identifier (DOI)

  • 10.1364/OPEX.13.003697

Citation Source

  • Scopus