Skip to main content

Data from: Finite-dimensional vestige of spinodal criticality above the dynamical glass transition

Publication ,  Dataset
Charbonneau, P; Kundu, J; Berthier, L
August 5, 2020

Finite-dimensional signatures of spinodal criticality are notoriously difficult to come by. The dynamical transition of glass-forming liquids, first described by mode-coupling theory, is a spinodal instability preempted by thermally activated processes that also limit how close the instability can be approached. We combine numerical tools to directly observe vestiges of the spinodal criticality in finite-dimensional glass formers. We use the swap Monte Carlo algorithm to efficiently thermalize configurations beyond the mode-coupling crossover, and analyze their dynamics using a scheme to screen out activated processes, in spatial dimensions ranging from d = 3 to d = 10. We observe a strong softening of the mean-field square-root singularity in d = 3 that is progressively restored as d increases above d = 8, in surprisingly good agreement with perturbation theory.

Duke Scholars

DOI

Publication Date

August 5, 2020
 

Citation

APA
Chicago
ICMJE
MLA
NLM
Charbonneau, P., Kundu, J., & Berthier, L. (2020). Data from: Finite-dimensional vestige of spinodal criticality above the dynamical glass transition. https://doi.org/10.7924/r4jh3m094
Charbonneau, Patrick, Joyjit Kundu, and Ludovic Berthier. “Data from: Finite-dimensional vestige of spinodal criticality above the dynamical glass transition,” August 5, 2020. https://doi.org/10.7924/r4jh3m094.
Charbonneau, Patrick, et al. Data from: Finite-dimensional vestige of spinodal criticality above the dynamical glass transition. 5 Aug. 2020. Manual, doi:10.7924/r4jh3m094.

DOI

Publication Date

August 5, 2020