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Local dynamical heterogeneity in glass formers

Publication ,  Journal Article
Biroli, G; Charbonneau, P; Folena, G; Hu, Y; Zamponi, F
Published in: Phys. Rev. Lett.
September 24, 2021

We study the local dynamical fluctuations in glass-forming models of particles embedded in $d$-dimensional space, in the mean-field limit of $d\to\infty$. Our analytical calculation reveals that single-particle observables, such as squared particle displacements, display divergent fluctuations around the dynamical (or mode-coupling) transition, due to the emergence of nontrivial correlations between displacements along different directions. This effect notably gives rise to a divergent non-Gaussian parameter, $\alpha_2$. The $d\to\infty$ local dynamics therefore becomes quite rich upon approaching the glass transition. The finite-$d$ remnant of this phenomenon further provides a long sought-after, first-principle explanation for the growth of $\alpha_2$ around the glass transition that is \emph{not based on multi-particle correlations}.

Duke Scholars

Published In

Phys. Rev. Lett.

Publication Date

September 24, 2021

Volume

128

Start / End Page

175501
 

Citation

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Biroli, G., Charbonneau, P., Folena, G., Hu, Y., & Zamponi, F. (2021). Local dynamical heterogeneity in glass formers. Phys. Rev. Lett., 128, 175501.
Biroli, Giulio, Patrick Charbonneau, Giampaolo Folena, Yi Hu, and Francesco Zamponi. “Local dynamical heterogeneity in glass formers.” Phys. Rev. Lett. 128 (September 24, 2021): 175501.
Biroli G, Charbonneau P, Folena G, Hu Y, Zamponi F. Local dynamical heterogeneity in glass formers. Phys Rev Lett. 2021 Sep 24;128:175501.
Biroli, Giulio, et al. “Local dynamical heterogeneity in glass formers.” Phys. Rev. Lett., vol. 128, Sept. 2021, p. 175501.
Biroli G, Charbonneau P, Folena G, Hu Y, Zamponi F. Local dynamical heterogeneity in glass formers. Phys Rev Lett. 2021 Sep 24;128:175501.

Published In

Phys. Rev. Lett.

Publication Date

September 24, 2021

Volume

128

Start / End Page

175501