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Spectroscopic demonstration of picosecond, phase-shifted laser multiple-pulse sequences

Publication ,  Journal Article
Spzno, F; Haner, M; Warren, WS
Published in: Chemical Physics Letters
March 27, 1987

We show that the concept of phase-shifted laser pulse trains is meaningful only for purely amplitude-modulated pulses, and probably cannot be generalized to use the output of a normal pulsed laser. We demonstrate a laser system which gives picosecond pulse lengths, picosecond or nanosecond interpulse delays, and complete phase control. This makes most molecular transitions amenable to the coherent techniques previously restricted to nuclear magnetic resonance. Fluorescence suppression by π phase shifts is demonstrated for the first time with picosecond pulses and long delays. © 1987.

Duke Scholars

Published In

Chemical Physics Letters

DOI

ISSN

0009-2614

Publication Date

March 27, 1987

Volume

135

Issue

1-2

Start / End Page

97 / 102

Related Subject Headings

  • Chemical Physics
  • 10 Technology
  • 03 Chemical Sciences
  • 02 Physical Sciences
 

Citation

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ICMJE
MLA
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Spzno, F., Haner, M., & Warren, W. S. (1987). Spectroscopic demonstration of picosecond, phase-shifted laser multiple-pulse sequences. Chemical Physics Letters, 135(1–2), 97–102. https://doi.org/10.1016/0009-2614(87)87224-X
Spzno, F., M. Haner, and W. S. Warren. “Spectroscopic demonstration of picosecond, phase-shifted laser multiple-pulse sequences.” Chemical Physics Letters 135, no. 1–2 (March 27, 1987): 97–102. https://doi.org/10.1016/0009-2614(87)87224-X.
Spzno F, Haner M, Warren WS. Spectroscopic demonstration of picosecond, phase-shifted laser multiple-pulse sequences. Chemical Physics Letters. 1987 Mar 27;135(1–2):97–102.
Spzno, F., et al. “Spectroscopic demonstration of picosecond, phase-shifted laser multiple-pulse sequences.” Chemical Physics Letters, vol. 135, no. 1–2, Mar. 1987, pp. 97–102. Scopus, doi:10.1016/0009-2614(87)87224-X.
Spzno F, Haner M, Warren WS. Spectroscopic demonstration of picosecond, phase-shifted laser multiple-pulse sequences. Chemical Physics Letters. 1987 Mar 27;135(1–2):97–102.
Journal cover image

Published In

Chemical Physics Letters

DOI

ISSN

0009-2614

Publication Date

March 27, 1987

Volume

135

Issue

1-2

Start / End Page

97 / 102

Related Subject Headings

  • Chemical Physics
  • 10 Technology
  • 03 Chemical Sciences
  • 02 Physical Sciences