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All-ultraviolet time-resolved coherent anti-Stokes Raman scattering

Publication ,  Journal Article
Mehendale, M; Giordmaine, JA; Gatzogiannis, E; Dogariu, A; Warren, WS; Beadie, G; Scully, MO
Published in: Optics Letters
January 15, 2006

We report all-UV coherent anti-Stokes Raman scattering (CARS) in calcite with 250-280 nm pump, Stokes, probe, and anti-Stokes light. UV CARS efficiency is ∼7X higher than for comparable scattering in the visible, 480-540 nm. Time-resolved UV CARS reveals lengthening of the dephasing time of 1086 cm -1 CO32- internal vibrations from 4 to 7 ps with increasing vibrational excitation, consistent with a phonon depletion model. © 2006 Optical Society of America.

Duke Scholars

Published In

Optics Letters

DOI

ISSN

0146-9592

Publication Date

January 15, 2006

Volume

31

Issue

2

Start / End Page

256 / 258

Related Subject Headings

  • Optics
  • 0906 Electrical and Electronic Engineering
  • 0206 Quantum Physics
  • 0205 Optical Physics
 

Citation

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Mehendale, M., Giordmaine, J. A., Gatzogiannis, E., Dogariu, A., Warren, W. S., Beadie, G., & Scully, M. O. (2006). All-ultraviolet time-resolved coherent anti-Stokes Raman scattering. Optics Letters, 31(2), 256–258. https://doi.org/10.1364/OL.31.000256
Mehendale, M., J. A. Giordmaine, E. Gatzogiannis, A. Dogariu, W. S. Warren, G. Beadie, and M. O. Scully. “All-ultraviolet time-resolved coherent anti-Stokes Raman scattering.” Optics Letters 31, no. 2 (January 15, 2006): 256–58. https://doi.org/10.1364/OL.31.000256.
Mehendale M, Giordmaine JA, Gatzogiannis E, Dogariu A, Warren WS, Beadie G, et al. All-ultraviolet time-resolved coherent anti-Stokes Raman scattering. Optics Letters. 2006 Jan 15;31(2):256–8.
Mehendale, M., et al. “All-ultraviolet time-resolved coherent anti-Stokes Raman scattering.” Optics Letters, vol. 31, no. 2, Jan. 2006, pp. 256–58. Scopus, doi:10.1364/OL.31.000256.
Mehendale M, Giordmaine JA, Gatzogiannis E, Dogariu A, Warren WS, Beadie G, Scully MO. All-ultraviolet time-resolved coherent anti-Stokes Raman scattering. Optics Letters. 2006 Jan 15;31(2):256–258.
Journal cover image

Published In

Optics Letters

DOI

ISSN

0146-9592

Publication Date

January 15, 2006

Volume

31

Issue

2

Start / End Page

256 / 258

Related Subject Headings

  • Optics
  • 0906 Electrical and Electronic Engineering
  • 0206 Quantum Physics
  • 0205 Optical Physics