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Identifying Life Cycle Environmental Hotspots in Phosphorus Recovery from Wastewater Using Modified Biochars

Publication ,  Journal Article
Zheng, X; Yan, G; Wang, X; Lam, KL
Published in: ACS Sustainable Chemistry and Engineering
November 25, 2024

Biochar offers a potential sustainable pathway for recovering phosphorus from wastewater to agriculture. Magnesium-modified biochar has demonstrated an enhanced phosphate adsorption capacity and excellent bioavailability. This study aims to identify the life cycle environmental hotspots in phosphorus recovery from wastewater using magnesium-modified biochars derived from bamboo, corn, and wood and compared them with common phosphate fertilizers. The results show that the biomass supply stage and the modification stage are the main environmental hotspots in most impact categories. As the phosphorus load of wastewater decreases, the phosphorus recovery stage could become the hotspot. Although phosphate-loaded magnesium-modified biochars in the base case do not have a better overall environmental performance than most phosphate fertilizers (especially those without nitrogen), they have significantly lower mineral resource scarcity and ecotoxicity. The sensitivity analysis suggests that the results are sensitive to the background inventory selected. The analysis indicates that the biochar yield, the phosphate adsorption capacity of the biochars, the source of modification chemical, and the source of biomass feedstock are key areas for technological and inventory improvement. In the future, a comprehensive field application inventory and a diverse set of background inventory are needed to better assess this sorption-based phosphorus recovery pathway.

Duke Scholars

Published In

ACS Sustainable Chemistry and Engineering

DOI

EISSN

2168-0485

Publication Date

November 25, 2024

Volume

12

Issue

47

Start / End Page

17319 / 17327

Related Subject Headings

  • 4004 Chemical engineering
  • 3401 Analytical chemistry
  • 0904 Chemical Engineering
  • 0502 Environmental Science and Management
  • 0301 Analytical Chemistry
 

Citation

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Zheng, X., Yan, G., Wang, X., & Lam, K. L. (2024). Identifying Life Cycle Environmental Hotspots in Phosphorus Recovery from Wastewater Using Modified Biochars. ACS Sustainable Chemistry and Engineering, 12(47), 17319–17327. https://doi.org/10.1021/acssuschemeng.4c07048
Zheng, X., G. Yan, X. Wang, and K. L. Lam. “Identifying Life Cycle Environmental Hotspots in Phosphorus Recovery from Wastewater Using Modified Biochars.” ACS Sustainable Chemistry and Engineering 12, no. 47 (November 25, 2024): 17319–27. https://doi.org/10.1021/acssuschemeng.4c07048.
Zheng X, Yan G, Wang X, Lam KL. Identifying Life Cycle Environmental Hotspots in Phosphorus Recovery from Wastewater Using Modified Biochars. ACS Sustainable Chemistry and Engineering. 2024 Nov 25;12(47):17319–27.
Zheng, X., et al. “Identifying Life Cycle Environmental Hotspots in Phosphorus Recovery from Wastewater Using Modified Biochars.” ACS Sustainable Chemistry and Engineering, vol. 12, no. 47, Nov. 2024, pp. 17319–27. Scopus, doi:10.1021/acssuschemeng.4c07048.
Zheng X, Yan G, Wang X, Lam KL. Identifying Life Cycle Environmental Hotspots in Phosphorus Recovery from Wastewater Using Modified Biochars. ACS Sustainable Chemistry and Engineering. 2024 Nov 25;12(47):17319–17327.
Journal cover image

Published In

ACS Sustainable Chemistry and Engineering

DOI

EISSN

2168-0485

Publication Date

November 25, 2024

Volume

12

Issue

47

Start / End Page

17319 / 17327

Related Subject Headings

  • 4004 Chemical engineering
  • 3401 Analytical chemistry
  • 0904 Chemical Engineering
  • 0502 Environmental Science and Management
  • 0301 Analytical Chemistry