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Theoretical study of the adsorption of H on Si n clusters, (n=3-10).

Publication ,  Journal Article
Tiznado, W; Oña, OB; Bazterra, VE; Caputo, MC; Facelli, JC; Ferraro, MB; Fuentealba, P
Published in: J Chem Phys
December 1, 2005

A recently proposed local Fukui function is used to predict the binding site of atomic hydrogen on silicon clusters. To validate the predictions, an extensive search for the more stable SinH (n=3-10) clusters has been done using a modified genetic algorithm. In all cases, the isomer predicted by the Fukui function is found by the search, but it is not always the most stable one. It is discussed that in the cases where the geometrical structure of the bare silicon cluster suffers a considerable change due to the addition of one hydrogen atom, the situation is more complicated and the relaxation effects should be considered.

Duke Scholars

Published In

J Chem Phys

DOI

ISSN

0021-9606

Publication Date

December 1, 2005

Volume

123

Issue

21

Start / End Page

214302

Location

United States

Related Subject Headings

  • Silicon
  • Models, Theoretical
  • Hydrogen
  • Chemical Physics
  • Binding Sites
  • Algorithms
  • Adsorption
  • 51 Physical sciences
  • 40 Engineering
  • 34 Chemical sciences
 

Citation

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Tiznado, W., Oña, O. B., Bazterra, V. E., Caputo, M. C., Facelli, J. C., Ferraro, M. B., & Fuentealba, P. (2005). Theoretical study of the adsorption of H on Si n clusters, (n=3-10). J Chem Phys, 123(21), 214302. https://doi.org/10.1063/1.2128675
Tiznado, William, Ofelia B. Oña, Víctor E. Bazterra, María C. Caputo, Julio C. Facelli, Marta B. Ferraro, and Patricio Fuentealba. “Theoretical study of the adsorption of H on Si n clusters, (n=3-10).J Chem Phys 123, no. 21 (December 1, 2005): 214302. https://doi.org/10.1063/1.2128675.
Tiznado W, Oña OB, Bazterra VE, Caputo MC, Facelli JC, Ferraro MB, et al. Theoretical study of the adsorption of H on Si n clusters, (n=3-10). J Chem Phys. 2005 Dec 1;123(21):214302.
Tiznado, William, et al. “Theoretical study of the adsorption of H on Si n clusters, (n=3-10).J Chem Phys, vol. 123, no. 21, Dec. 2005, p. 214302. Pubmed, doi:10.1063/1.2128675.
Tiznado W, Oña OB, Bazterra VE, Caputo MC, Facelli JC, Ferraro MB, Fuentealba P. Theoretical study of the adsorption of H on Si n clusters, (n=3-10). J Chem Phys. 2005 Dec 1;123(21):214302.

Published In

J Chem Phys

DOI

ISSN

0021-9606

Publication Date

December 1, 2005

Volume

123

Issue

21

Start / End Page

214302

Location

United States

Related Subject Headings

  • Silicon
  • Models, Theoretical
  • Hydrogen
  • Chemical Physics
  • Binding Sites
  • Algorithms
  • Adsorption
  • 51 Physical sciences
  • 40 Engineering
  • 34 Chemical sciences