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Zero-temperature glass transition in two dimensions.

Publication ,  Journal Article
Berthier, L; Charbonneau, P; Ninarello, A; Ozawa, M; Yaida, S
Published in: Nature communications
April 2019

Liquids cooled towards the glass transition temperature transform into amorphous solids that have a wide range of applications. While the nature of this transformation is understood rigorously in the mean-field limit of infinite spatial dimensions, the problem remains wide open in physical dimensions. Nontrivial finite-dimensional fluctuations are hard to control analytically, and experiments fail to provide conclusive evidence regarding the nature of the glass transition. Here, we develop Monte Carlo methods for two-dimensional glass-forming liquids that allow us to access equilibrium states at sufficiently low temperatures to directly probe the glass transition in a regime inaccessible to experiments. We find that the liquid state terminates at a thermodynamic glass transition which occurs at zero temperature and is associated with an entropy crisis and a diverging static correlation length. Our results thus demonstrate that a thermodynamic glass transition can occur in finite dimensional glass-formers.

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Published In

Nature communications

DOI

EISSN

2041-1723

ISSN

2041-1723

Publication Date

April 2019

Volume

10

Issue

1

Start / End Page

1508
 

Citation

APA
Chicago
ICMJE
MLA
NLM
Berthier, L., Charbonneau, P., Ninarello, A., Ozawa, M., & Yaida, S. (2019). Zero-temperature glass transition in two dimensions. Nature Communications, 10(1), 1508. https://doi.org/10.1038/s41467-019-09512-3
Berthier, Ludovic, Patrick Charbonneau, Andrea Ninarello, Misaki Ozawa, and Sho Yaida. “Zero-temperature glass transition in two dimensions.Nature Communications 10, no. 1 (April 2019): 1508. https://doi.org/10.1038/s41467-019-09512-3.
Berthier L, Charbonneau P, Ninarello A, Ozawa M, Yaida S. Zero-temperature glass transition in two dimensions. Nature communications. 2019 Apr;10(1):1508.
Berthier, Ludovic, et al. “Zero-temperature glass transition in two dimensions.Nature Communications, vol. 10, no. 1, Apr. 2019, p. 1508. Epmc, doi:10.1038/s41467-019-09512-3.
Berthier L, Charbonneau P, Ninarello A, Ozawa M, Yaida S. Zero-temperature glass transition in two dimensions. Nature communications. 2019 Apr;10(1):1508.

Published In

Nature communications

DOI

EISSN

2041-1723

ISSN

2041-1723

Publication Date

April 2019

Volume

10

Issue

1

Start / End Page

1508