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Mean-Field Caging in a Random Lorentz Gas.

Publication ,  Journal Article
Biroli, G; Charbonneau, P; Hu, Y; Ikeda, H; Szamel, G; Zamponi, F
Published in: The journal of physical chemistry. B
June 2021

The random Lorentz gas (RLG) is a minimal model of both percolation and glassiness, which leads to a paradox in the infinite-dimensional, d → ∞ limit: the localization transition is then expected to be continuous for the former and discontinuous for the latter. As a putative resolution, we have recently suggested that, as d increases, the behavior of the RLG converges to the glassy description and that percolation physics is recovered thanks to finite-d perturbative and nonperturbative (instantonic) corrections [Biroli et al. Phys. Rev. E 2021, 103, L030104]. Here, we expand on the d → ∞ physics by considering a simpler static solution as well as the dynamical solution of the RLG. Comparing the 1/d correction of this solution with numerical results reveals that even perturbative corrections fall out of reach of existing theoretical descriptions. Comparing the dynamical solution with the mode-coupling theory (MCT) results further reveals that, although key quantitative features of MCT are far off the mark, it does properly capture the discontinuous nature of the d → ∞ RLG. These insights help chart a path toward a complete description of finite-dimensional glasses.

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Published In

The journal of physical chemistry. B

DOI

EISSN

1520-5207

ISSN

1520-6106

Publication Date

June 2021

Volume

125

Issue

23

Start / End Page

6244 / 6254

Related Subject Headings

  • 51 Physical sciences
  • 40 Engineering
  • 34 Chemical sciences
  • 09 Engineering
  • 03 Chemical Sciences
  • 02 Physical Sciences
 

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Biroli, G., Charbonneau, P., Hu, Y., Ikeda, H., Szamel, G., & Zamponi, F. (2021). Mean-Field Caging in a Random Lorentz Gas. The Journal of Physical Chemistry. B, 125(23), 6244–6254. https://doi.org/10.1021/acs.jpcb.1c02067
Biroli, Giulio, Patrick Charbonneau, Yi Hu, Harukuni Ikeda, Grzegorz Szamel, and Francesco Zamponi. “Mean-Field Caging in a Random Lorentz Gas.The Journal of Physical Chemistry. B 125, no. 23 (June 2021): 6244–54. https://doi.org/10.1021/acs.jpcb.1c02067.
Biroli G, Charbonneau P, Hu Y, Ikeda H, Szamel G, Zamponi F. Mean-Field Caging in a Random Lorentz Gas. The journal of physical chemistry B. 2021 Jun;125(23):6244–54.
Biroli, Giulio, et al. “Mean-Field Caging in a Random Lorentz Gas.The Journal of Physical Chemistry. B, vol. 125, no. 23, June 2021, pp. 6244–54. Epmc, doi:10.1021/acs.jpcb.1c02067.
Biroli G, Charbonneau P, Hu Y, Ikeda H, Szamel G, Zamponi F. Mean-Field Caging in a Random Lorentz Gas. The journal of physical chemistry B. 2021 Jun;125(23):6244–6254.
Journal cover image

Published In

The journal of physical chemistry. B

DOI

EISSN

1520-5207

ISSN

1520-6106

Publication Date

June 2021

Volume

125

Issue

23

Start / End Page

6244 / 6254

Related Subject Headings

  • 51 Physical sciences
  • 40 Engineering
  • 34 Chemical sciences
  • 09 Engineering
  • 03 Chemical Sciences
  • 02 Physical Sciences