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Propagation effects on the peak profile in two-dimensional optical photon echo spectroscopy

Publication ,  Journal Article
Keusters, D; Warren, WS
Published in: Chemical Physics Letters
January 1, 2004

The effect of pulse propagation on the lineshape in a two-dimensional photon echo spectrum is investigated using the coupled Maxwell Bloch equations. Reshaping of excitation and signal pulses due to propagation results in broadening of peak profiles. The amount of broadening is not symmetric along the two dimensions and depends on pulse intensity and relaxation mechanism. It is found that relaxation mechanisms that give the same lineshape at low optical density (OD) can give different lineshapes at high OD. Even at relatively low OD the reshaping can be quite severe, and might result in misinterpretation of the obtained spectrum. © 2003 Published by Elsevier B.V.

Duke Scholars

Published In

Chemical Physics Letters

DOI

ISSN

0009-2614

Publication Date

January 1, 2004

Volume

383

Issue

1-2

Start / End Page

21 / 24

Related Subject Headings

  • Chemical Physics
  • 10 Technology
  • 03 Chemical Sciences
  • 02 Physical Sciences
 

Citation

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Keusters, D., & Warren, W. S. (2004). Propagation effects on the peak profile in two-dimensional optical photon echo spectroscopy. Chemical Physics Letters, 383(1–2), 21–24. https://doi.org/10.1016/j.cplett.2003.10.130
Keusters, D., and W. S. Warren. “Propagation effects on the peak profile in two-dimensional optical photon echo spectroscopy.” Chemical Physics Letters 383, no. 1–2 (January 1, 2004): 21–24. https://doi.org/10.1016/j.cplett.2003.10.130.
Keusters D, Warren WS. Propagation effects on the peak profile in two-dimensional optical photon echo spectroscopy. Chemical Physics Letters. 2004 Jan 1;383(1–2):21–4.
Keusters, D., and W. S. Warren. “Propagation effects on the peak profile in two-dimensional optical photon echo spectroscopy.” Chemical Physics Letters, vol. 383, no. 1–2, Jan. 2004, pp. 21–24. Scopus, doi:10.1016/j.cplett.2003.10.130.
Keusters D, Warren WS. Propagation effects on the peak profile in two-dimensional optical photon echo spectroscopy. Chemical Physics Letters. 2004 Jan 1;383(1–2):21–24.
Journal cover image

Published In

Chemical Physics Letters

DOI

ISSN

0009-2614

Publication Date

January 1, 2004

Volume

383

Issue

1-2

Start / End Page

21 / 24

Related Subject Headings

  • Chemical Physics
  • 10 Technology
  • 03 Chemical Sciences
  • 02 Physical Sciences