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Effect of pulse propagation on the two-dimensional photon echo spectrum of multilevel systems

Publication ,  Journal Article
Keusters, D; Warren, WS
Published in: Journal of Chemical Physics
August 22, 2003

A perturbative method was used to investigate the effect of propagation on multilevel systems, specifically on the relative intensity and profile of the cross peaks. It was shown that both the peak profiles and the relative intensity of the peaks in a 2D spectrum change as the pulse propagates through the sample. The behavior of the peaks was found to be counterintuitive, and depends not only on the optical density, but also on the dynamics of the system.

Duke Scholars

Published In

Journal of Chemical Physics

DOI

ISSN

0021-9606

Publication Date

August 22, 2003

Volume

119

Issue

8

Start / End Page

4478 / 4489

Related Subject Headings

  • Chemical Physics
  • 51 Physical sciences
  • 40 Engineering
  • 34 Chemical sciences
  • 09 Engineering
  • 03 Chemical Sciences
  • 02 Physical Sciences
 

Citation

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MLA
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Keusters, D., & Warren, W. S. (2003). Effect of pulse propagation on the two-dimensional photon echo spectrum of multilevel systems. Journal of Chemical Physics, 119(8), 4478–4489. https://doi.org/10.1063/1.1591175
Keusters, D., and W. S. Warren. “Effect of pulse propagation on the two-dimensional photon echo spectrum of multilevel systems.” Journal of Chemical Physics 119, no. 8 (August 22, 2003): 4478–89. https://doi.org/10.1063/1.1591175.
Keusters D, Warren WS. Effect of pulse propagation on the two-dimensional photon echo spectrum of multilevel systems. Journal of Chemical Physics. 2003 Aug 22;119(8):4478–89.
Keusters, D., and W. S. Warren. “Effect of pulse propagation on the two-dimensional photon echo spectrum of multilevel systems.” Journal of Chemical Physics, vol. 119, no. 8, Aug. 2003, pp. 4478–89. Scopus, doi:10.1063/1.1591175.
Keusters D, Warren WS. Effect of pulse propagation on the two-dimensional photon echo spectrum of multilevel systems. Journal of Chemical Physics. 2003 Aug 22;119(8):4478–4489.

Published In

Journal of Chemical Physics

DOI

ISSN

0021-9606

Publication Date

August 22, 2003

Volume

119

Issue

8

Start / End Page

4478 / 4489

Related Subject Headings

  • Chemical Physics
  • 51 Physical sciences
  • 40 Engineering
  • 34 Chemical sciences
  • 09 Engineering
  • 03 Chemical Sciences
  • 02 Physical Sciences