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Selective excitation of high vibrational states using Raman chirped adiabatic passage

Publication ,  Journal Article
Davis, JC; Warren, WS
Published in: Journal of Chemical Physics
March 1, 1999

Calculations indicate that high vibrational states of oxygen and chlorine can be excited using a series of nonresonant Raman pulses, where both the pump and the Stokes pulses are chirped with linear frequency sweeps. Most of the previously reported coherent processes (such as simple adiabatic passage) are seriously degraded when rotational effects are included. However, we find that the laser pulse parameters (intensity and bandwidth) required to invert population into high vibrational states via Raman chirped adiabatic passage are achievable using technology that is currently available. Applications to homonuclear diatomic molecules are discussed in detail. © 1999 American Institute of Physics.

Duke Scholars

Published In

Journal of Chemical Physics

DOI

ISSN

0021-9606

Publication Date

March 1, 1999

Volume

110

Issue

9

Start / End Page

4229 / 4237

Related Subject Headings

  • Chemical Physics
  • 51 Physical sciences
  • 40 Engineering
  • 34 Chemical sciences
  • 09 Engineering
  • 03 Chemical Sciences
  • 02 Physical Sciences
 

Citation

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MLA
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Davis, J. C., & Warren, W. S. (1999). Selective excitation of high vibrational states using Raman chirped adiabatic passage. Journal of Chemical Physics, 110(9), 4229–4237. https://doi.org/10.1063/1.478305
Davis, J. C., and W. S. Warren. “Selective excitation of high vibrational states using Raman chirped adiabatic passage.” Journal of Chemical Physics 110, no. 9 (March 1, 1999): 4229–37. https://doi.org/10.1063/1.478305.
Davis JC, Warren WS. Selective excitation of high vibrational states using Raman chirped adiabatic passage. Journal of Chemical Physics. 1999 Mar 1;110(9):4229–37.
Davis, J. C., and W. S. Warren. “Selective excitation of high vibrational states using Raman chirped adiabatic passage.” Journal of Chemical Physics, vol. 110, no. 9, Mar. 1999, pp. 4229–37. Scopus, doi:10.1063/1.478305.
Davis JC, Warren WS. Selective excitation of high vibrational states using Raman chirped adiabatic passage. Journal of Chemical Physics. 1999 Mar 1;110(9):4229–4237.

Published In

Journal of Chemical Physics

DOI

ISSN

0021-9606

Publication Date

March 1, 1999

Volume

110

Issue

9

Start / End Page

4229 / 4237

Related Subject Headings

  • Chemical Physics
  • 51 Physical sciences
  • 40 Engineering
  • 34 Chemical sciences
  • 09 Engineering
  • 03 Chemical Sciences
  • 02 Physical Sciences